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Friedrich-Schiller-Universitat Jena QED 2005 Les Houches

Casimir-Polder forces
between atoms and
magnetodielectric bodies
Stefan Yoshi Buhmann and Dirk-Gunnar Welsch
Theoretisch-Physikalisches Institut
Friedrich-Schiller-Universitat Jena, Germany
Electronic address: s.buhmann@tpi.uni-jena.de
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Puzzle
What is greater than God,
more evil than the devil?
The poor have it,
the happy need it,
and if you eat it, you will die.
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Puzzle
What is greater than God,
more evil than the devil?
The poor have it,
the happy need it,
and if you eat it, you will die.
Answer: Nothing
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Content
Introduction
QED vacuum and induced forces
Duality in the context of vacuum forces
Motivation
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Content
Introduction
QED vacuum and induced forces
Duality in the context of vacuum forces
Motivation
General Theory
Quantization scheme
Perturbative Casimir-Polder force
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Content
Introduction
QED vacuum and induced forces
Duality in the context of vacuum forces
Motivation
General Theory
Quantization scheme
Perturbative Casimir-Polder force
Recent results: Casimir-Polder force
Specic examples: half space, plate, planar cavity
Born expansion of the Casimir-Polder force
Microscopic origin of the Casimir-Polder force
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Content
Introduction
QED vacuum and induced forces
Duality in the context of vacuum forces
Motivation
General Theory
Quantization scheme
Perturbative Casimir-Polder force
Recent results: Casimir-Polder force
Specic examples: half space, plate, planar cavity
Born expansion of the Casimir-Polder force
Microscopic origin of the Casimir-Polder force
Summary and outlook
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
The QED vacuum
vacuus [lat.]: empty
Classical electrodynamics:
E
n
(r)) = 0, B
n
(r)) = 0 n (no electromagnetic eld)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
The QED vacuum
vacuus [lat.]: empty
Classical electrodynamics:
E
n
(r)) = 0, B
n
(r)) = 0 n (no electromagnetic eld)
QED: [
0

E
i
(r),

B
j
(r
t
)] = i
ijk

k
(r r
t
)
AB
1
2
[[

A,

B])[ (Heisenberg uncertainty relation)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
The QED vacuum
vacuus [lat.]: empty
Classical electrodynamics:
E
n
(r)) = 0, B
n
(r)) = 0 n (no electromagnetic eld)
QED: [
0

E
i
(r),

B
j
(r
t
)] = i
ijk

k
(r r
t
)
AB
1
2
[[

A,

B])[ (Heisenberg uncertainty relation)

QED vacuum: [E
(+)
(r)]
n
) = 0, [B
(+)
(r)]
n
) = 0 n

E(r)) = 0,

B(r)) = 0 (no e.m. eld on average)


but: E(r) ,= 0, B(r) ,= 0 (eld uctuations)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Vacuum forces
Field uctuations
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Vacuum forces
Field uctuations Forces on polarizable objects:
atom atom (van der Waals/Casimir-Polder force)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Vacuum forces
Field uctuations Forces on polarizable objects:
atom atom (van der Waals/Casimir-Polder force)
atom body (van der Waals/Casimir-Polder force)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Vacuum forces
Field uctuations Forces on polarizable objects:
atom atom (van der Waals/Casimir-Polder force)
atom body (van der Waals/Casimir-Polder force)
body body (Casimir force)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Forces and duality
+ +
_ _
1. Two electrically polarizable objects (
e

e
):
attractive force
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Forces and duality
+ +
_ _
1. Two electrically polarizable objects (
e

e
):
attractive force
Duality transformation: Absence of free charges/currents
theory invariant under transformation E

B (
e


m
)

Friedrich-Schiller-Universitat Jena QED 2005 Les Houches


Forces and duality
N N S S
1. Two electrically polarizable objects (
e

e
):
attractive force
Duality transformation: Absence of free charges/currents
theory invariant under transformation E

B (
e


m
)

2. Two magnetically polarizable objects (


m

m
):
attractive force
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Forces and duality
N + S
_
1. Two electrically polarizable objects (
e

e
):
attractive force
Duality transformation: Absence of free charges/currents
theory invariant under transformation E

B (
e


m
)

2. Two magnetically polarizable objects (


m

m
):
attractive force
3. Two objects of opposed polarizability (
e

m
):
No duality transformation, repulsive force
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Forces and duality
1. Two electrically polarizable objects (
e

e
):
attractive force
Duality transformation: Absence of free charges/currents
theory invariant under transformation E

B (
e


m
)

2. Two magnetically polarizable objects (


m

m
):
attractive force
3. Two objects of opposed polarizability (
e

m
):
No duality transformation, repulsive force
Question: Atom magnetodielectric body?
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Casimir-Polder force:
Atom magnetodielectric bodies
Practical aspects
Measurement: Accurate methods available
Nuisance: Nanotechnology lifetime above atom chip
Potential: Atom optics design of nanostructures
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Casimir-Polder force:
Atom magnetodielectric bodies
Practical aspects
Measurement: Accurate methods available
Nuisance: Nanotechnology lifetime above atom chip
Potential: Atom optics design of nanostructures
+
Magnetodielectrics
Material design: Controllable electromagnetic properties
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Casimir-Polder force:
Atom magnetodielectric bodies
Practical aspects
Measurement: Accurate methods available
Nuisance: Nanotechnology lifetime above atom chip
Potential: Atom optics design of nanostructures
+
Magnetodielectrics
Material design: Controllable electromagnetic properties
+
Fundamental aspects
Duality: Electric vs magnetic medium properties
Born expansion: Additivity, microscopic origin
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Casimir-Polder force:
Atom magnetodielectric bodies
Practical aspects
Measurement: Accurate methods available
Nuisance: Nanotechnology lifetime above atom chip
Potential: Atom optics design of nanostructures
+
Magnetodielectrics
Material design: Controllable electromagnetic properties
+
Fundamental aspects
Duality: Electric vs magnetic medium properties
Born expansion: Additivity, microscopic origin

Casimir-Polder force: Atom magnetodielectric bodies


Future perspective: Potential engineering and control
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Central Issues
Casimir-Polder force:
Ground-state atom magnetodielectric bodies
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Central Issues
Casimir-Polder force:
Ground-state atom magnetodielectric bodies
Sign and strength of force
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Central Issues
Casimir-Polder force:
Ground-state atom magnetodielectric bodies
Sign and strength of force
Dependence on geometric parameters
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Central Issues
+ + +
Casimir-Polder force:
Ground-state atom magnetodielectric bodies
Sign and strength of force
Dependence on geometric parameters
Additivity
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Central Issues
+ + +
Casimir-Polder force:
Ground-state atom magnetodielectric bodies
Sign and strength of force
Dependence on geometric parameters
Additivity
Microscopic origin
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Quantization scheme
Normal-mode quantization of electric eld:

E(r) =

k
g
k
(r)a
k
+H.c.

c-number functions

creation/annihilation
operators

Friedrich-Schiller-Universitat Jena QED 2005 Les Houches


Quantization scheme
Normal-mode quantization of electric eld:

E(r) =

k
g
k
(r)a
k
+H.c.

c-number functions

creation/annihilation
operators

Quantized electric eld in linear, causal media:

E(r) =
_

0
d
_
d
3
r
t
i

0
_

2
c
2
_
Im(r
t
, ) G(r, r
t
, )

f
e
(r
t
, )
+

c
_
Im
1
(r
t
, )
_

t
G(r, r
t
, )
_

f
m
(r
t
, )
_
+H.c.
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Atom-eld dynamics

H =

H
MF
+

H
A
+

H
AMF
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Atom-eld dynamics

H =

H
MF
+

H
A
+

H
AMF
Medium-assisted eld Hamiltonian:

H
MF
=

=e,m
_
d
3
r
_

0
d

(r, )

(r, )
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Atom-eld dynamics

H =

H
MF
+

H
A
+

H
AMF
Medium-assisted eld Hamiltonian:

H
MF
=

=e,m
_
d
3
r
_

0
d

(r, )

(r, )
Atomic Hamiltonian:

H
A
=

2
2m

+
1
2
0
_
d
3
r

P
A
2
(r)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Atom-eld dynamics

H =

H
MF
+

H
A
+

H
AMF
Medium-assisted eld Hamiltonian:

H
MF
=

=e,m
_
d
3
r
_

0
d

(r, )

(r, )
Atomic Hamiltonian:

H
A
=

2
2m

+
1
2
0
_
d
3
r

P
A
2
(r)
Electric dipole interaction:

H
AMF
=

E(r
A
) +
1
2m
A
_
p
A
,

d

B(r
A
)
_
+
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Ground-state CP force
Idea: System in state [0) [0) ,
Interaction

H
AMF
energy shift E
0
van-der-Waals potential E
0
= E
(0)
0
+U(r
A
)
Casimir-Polder force F(r
A
) =
A
U(r
A
)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Ground-state CP force
Idea: System in state [0) [0) ,
Interaction

H
AMF
energy shift E
0
van-der-Waals potential E
0
= E
(0)
0
+U(r
A
)
Casimir-Polder force F(r
A
) =
A
U(r
A
)
2
nd
-order perturbation theory:
2
E
0
=

[0[0[

H
AMF
[)[
2
E
0
E

Friedrich-Schiller-Universitat Jena QED 2005 Les Houches


Ground-state CP force
Idea: System in state [0) [0) ,
Interaction

H
AMF
energy shift E
0
van-der-Waals potential E
0
= E
(0)
0
+U(r
A
)
Casimir-Polder force F(r
A
) =
A
U(r
A
)
2
nd
-order perturbation theory:
2
E
0
=

[0[0[

H
AMF
[)[
2
E
0
E

Result:
U(r
A
) =

0
2
_

0
duu
2
(iu) TrG
(1)
(r
A
, r
A
, iu)
Atomic polarizability:
() = lim
0
2
3

k0
[d
0k
[
2

2
k0

2
i
Scattering Green
tensor:
G
(1)
(r
A
, r
A
, iu)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Atom near half space
1
A
z
() ( )
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Atom near half space
1
A
z
() ( )
Short distance: z
A
_ c/
+
M
, c/
+
A
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Atom near half space
1
A
z
()
Short distance: z
A
_ c/
+
M
, c/
+
A
Purely dielectric half space: U(z
A
) =
C
3
z
3
A
C
3
=

16
2

0
_

0
du(iu)
(iu) 1
(iu) +1
0
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Atom near half space
1
A
z
( )
Short distance: z
A
_ c/
+
M
, c/
+
A
Purely dielectric half space: U(z
A
) =
C
3
z
3
A
C
3
=

16
2

0
_

0
du(iu)
(iu) 1
(iu) +1
0
Purely magnetic half space: U(z
A
) = +
C
1
z
A
C
1
=

16
2

0
_

0
du
_
u
c
_
2
(iu)
_
(iu) 1
(iu) +1
+
(iu) 1
2
_
0
1
S.Y.B., Ho Trung Dung, T. Kampf, and D.G.W., EPJD, DOI:
10.1140/epjd/e2005-00044-6 (2005)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Atom near half space
Long distance: z
A
c/

M
, c/

A
U(z
A
) =
C
4
z
4
A
C
4
= C
4
[(0), (0), (0)] 0
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Atom near half space
Long distance: z
A
c/

M
, c/

A
U(z
A
) =
C
4
z
4
A
C
4
= C
4
[(0), (0), (0)] 0
1
3
5
7
9
11
1 1.5 2 2.5 3
(0)
(0)
repulsive
attractive
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Atom near half space
Numerical results: Two-level atom, Drude-Lorentz model
-0.0004
0
0.0004
0.0008
0 2 4 6 8 10
bar200.txt u 3:8
bar180.txt u 3:8
bar160.txt u 3:8
bar120.txt u 3:8
bar043.txt u 3:8
PSfrag replacements
z
A

Tm
/c
U
(
z
A
)
1
2

2
c
/
(

3 T
m
d
2 1
0
)

Pm
= 2.00

Pm
= 1.80

Pm
= 1.60

Pm
= 1.20

Pm
= 0.43
C
1
C
3
C
4
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Atom near plate
Numerical results: Two-level atom, Drude-Lorentz model
0
0.0004
0.0008
0.0012
2 4 6 8
PSfrag replacements
z
A

Tm
/c
U
(
z
A
)
1
2

2
c
/
(

3 T
m
d
2 1
0
)
d
10
/c =0.01
d
10
/c =0.10
d
10
/c =0.55
d
10
/c =1.50
d
10
/c =4.00
d
10
/c
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Relations between dispersion forces
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Relations between dispersion forces
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Relations between dispersion forces
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Born expansion of the vdW potential
Method: =1 +
expand G in powers of (Born series)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Born expansion of the vdW potential
Method: =1 +
expand G in powers of (Born series)
Result:
U(r
A
) =

k=1

k
U(r
A
)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Born expansion of the vdW potential
Method: =1 +
expand G in powers of (Born series)
Result:
U(r
A
) =

k=1

k
U(r
A
)

k
U(r
A
) =
()
k

0
2c
2k
_

0
duu
2k+2
(iu)
_
_
k

j=1
_
d
3
s
j
(iu, s
j
)
_
_
Tr [G
vac
(r
A
, s
1
, iu) G
vac
(s
1
, s
2
, iu) . . . G
vac
(s
k
, r
A
, iu)]
=
+ +
...

Friedrich-Schiller-Universitat Jena QED 2005 Les Houches


First order in : Additivity
(Half space + half space Planar cavity)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
First order in : Additivity
(Half space + half space Planar cavity)
1. Dielectric cavity:
+ =
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
First order in : Additivity
(Half space + half space Planar cavity)
1. Dielectric cavity:
+ =
2. Magnetic cavity:
+ =
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
First order in : Additivity
(Half space + half space Planar cavity)
1. Dielectric cavity:
+ =
2. Magnetic cavity:
+ =
3. Magnetodielectric cavity:
+ =
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Planar cavity
Numerical results: two-level atom, Drude-Lorentz model
PSfrag replacements
z
A

10
/c
U
(
z
A
)
1
2

0
c
3
/
(

3 1
0
|
d
0
1
|
2
)
(a)
(b)
(c)
0
0
5 10 15
0.002
0.001
0.001
0.002
electric
magnetic
d
i
e
l
e
c
t
r
i
c
m
a
g
n
e
t
o

Friedrich-Schiller-Universitat Jena QED 2005 Les Houches


Second order in : Correlations
(Thin plate Half space)
1
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Second order in : Correlations
(Thin plate Half space)
1

1
U(z
A
) +
2
U(z
A
) =
_

z
A
dz
d

1
U
d
(z) +
2
U
d
(z)
+
_

z
A
dz
d
_

0
ds
d

2
U
dd
(z
A
, s)
A
z
A
z
A
z
z
z s
=
+

1
S.Y.B., T. Kampf, and D.G.W., submitted to PRA
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Microscopic origin of the vdW potential
Dilute atomic gas: (r, ) =
1
0
n(r)()
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Microscopic origin of the vdW potential
Dilute atomic gas: (r, ) =
1
0
n(r)()
Result:
U(r
A
) =

k=1
1
k!
_
_
k

j=1
_
d
3
s
j
n(s
j
)
_
_
U(r
A
, s
1
, . . . , s
k
)
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Microscopic origin of the vdW potential
Dilute atomic gas: (r, ) =
1
0
n(r)()
Result:
U(r
A
) =

k=1
1
k!
_
_
k

j=1
_
d
3
s
j
n(s
j
)
_
_
U(r
A
, s
1
, . . . , s
k
)
U(r
1
, . . . , r
l
) =
()
l1

l
0
2l
_

0
duu
2l
[(iu)]
l

p
Tr
_
G
vac
(r
p(1)
, r
p(2)
, iu) . . . G
vac
(r
p(l)
, r
p(1)
, iu)
_
=
+ +
...

Friedrich-Schiller-Universitat Jena QED 2005 Les Houches


Summary
Dielectric half space: Attractive force
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Summary
Dielectric half space: Attractive force
Magnetic half space: Repulsive force
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Summary
Dielectric half space: Attractive force
Magnetic half space: Repulsive force
Magnetodielectric half space: Potential wall
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Summary
Dielectric half space: Attractive force
Magnetic half space: Repulsive force
Magnetodielectric half space: Potential wall
Plate thickness: Inuences height of wall
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Summary
Dielectric half space: Attractive force
Magnetic half space: Repulsive force
Magnetodielectric half space: Potential wall
Plate thickness: Inuences height of wall
Born expansion: Small bodies larger bodies
Half space + half space planar cavity
+ =
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Summary
Dielectric half space: Attractive force
Magnetic half space: Repulsive force
Magnetodielectric half space: Potential wall
Plate thickness: Inuences height of wall
Born expansion: Small bodies larger bodies
Half space + half space planar cavity
Thin plate half space
+
=

Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Summary
Dielectric half space: Attractive force
Magnetic half space: Repulsive force
Magnetodielectric half space: Potential wall
Plate thickness: Inuences height of wall
Born expansion: Small bodies larger bodies
Half space + half space planar cavity
Thin plate half space
Microscopic origin: Innite series of many-atom potentials
=
+ +
...
Friedrich-Schiller-Universitat Jena QED 2005 Les Houches
Summary
Dielectric half space: Attractive force
Magnetic half space: Repulsive force
Magnetodielectric half space: Potential wall
Plate thickness: Inuences height of wall
Born expansion: Small bodies larger bodies
Half space + half space planar cavity
Thin plate half space
Microscopic origin: Innite series of many-atom potentials
Outlook
Eects of surface roughness and small permittivity variations
Excited atom magnetodielectric bodies

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