Cinerica Quimia 1

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\cf0 Contribucin a la Educacin y la Proteccin Ambiental. Vol. 5. (2004) ISBN 959-71
36-24-4
\par}{\phpg\posx1623\pvpg\posy1144\absw7615\absh791 \sl-152 \par\i \f20 \fs17 \c
f0 \fi604 {\b\i0 \fs14 APLICACIONES}{\b\i0 \fs14 DE}{\b\i0 \fs14 LA}{\b\i0 \f
s14 CINTICA}{\b\i0 \fs14 EN}{\b\i0 \fs14 LA}{\b\i0 \fs14 HIDROGEOLOGA}{\b\i0
\fs14 Y}{\b\i0 \fs14 EL}{\b\i0 \fs14 MEDIO}{\b\i0 \fs14 AMBIENTE. }
f0 \fi3288 {\i0 \fs14 J.}{\i0 \fs14 R.}{\i0 \fs14 Fagundo,}{\i0 \fs14 et}{\i0
\fs14 al. }\par
}
{\phpg\posx9874\pvpg\posy1846\absw510\absh179 \f20 \fs16 \cf0 \f20 \fs16 \cf0 80
H \par
}
{\phpg\posx1181\pvpg\posy2299\absw10080\absh1254 \b \f20 \fs21 \cf0 \b \f20 \fs2
1 \cf0 APLICACIONES DE LA CINTICA EN LA HIDROGEOLOGA Y EL MEDIO AMBIENTE
\par}{\phpg\posx1181\pvpg\posy2299\absw10080\absh1254 \sl-280 \par\b \f20 \fs21
\cf0 \fi1499 {\b0\i J.}{\b0\i R.}{\b0\i Fagundo}{\b0\i\up006 \fs14 1}{\b0\i ,
}{\b0\i P.}{\b0\i Gonzlez}{\b0\i\up006 \fs14 1}{\b0\i ,}{\b0\i M.}{\b0\i Rod
rguez}{\b0\i\up006 \fs14 2}{\b0\i ,}{\b0\i M.}{\b0\i Surez}{\b0\i\up006 \fs14
1}{\b0\i ,}{\b0\i C.}{\b0\i Melin}{\b0\i\up006 \fs14 1 }
\par}{\phpg\posx1181\pvpg\posy2299\absw10080\absh1254 \sl-283 \par\b \f20 \fs21
\cf0 \fi628 {\b0\i\up006 \fs14 1}{\b0\i Centro}{\b0\i Nacional}{\b0\i de}{\b0\
i Medicina}{\b0\i Natural}{\b0\i y}{\b0\i Tradicional.}{\b0\i MINAP}{\b0\i
{\ul (}{\ul j}{\ul u}{\ul a}{\ul n}{\ul r}{\ul f}{\ul a}{\ul g}{\ul @}{\ul i}{\
ul n}{\ul f}{\ul o}{\ul m}{\ul e}{\ul d}{\ul .}{\ul s}{\ul l}{\ul d}{\ul .}{\ul
c}{\ul u}) }\par
}
{\phpg\posx2801\pvpg\posy3672\absw91\absh160 \i \f20 \fs14 \cf0 \i \f20 \fs14 \c
f0 2 \par
}
{\phpg\posx2943\pvpg\posy3710\absw7124\absh746 \i \f20 \fs21 \cf0 \i \f20 \fs21
\cf0 Centro de Estudios de Medio Ambiente. Universidad de La Habana
f0 \fi2592 {\b RESUMEN }\par
}
{\phpg\posx1136\pvpg\posy4785\absw10919\absh8892 \i \f20 \fs21 \cf0 \fi110 \i \f
20 \fs21 \cf0 En un trabajo anterior se trat sobre las aplicaciones termodinmicas
en la Hidrogeologa, donde se
\par}{\phpg\posx1136\pvpg\posy4785\absw10919\absh8892 \sl-283 \i \f20 \fs21 \cf0
\fi167 abordaron los fundamentos termodinmicos del equilibrio qumico y se ejempli
fic su aplicacin en
\fi184 problemas relacionados con la misma (Fagundo et al., 2003). En el presen
te trabajo se discuten los
\fi345 principios de la cintica y se muestra, mediante experimentos en el labora
torio y en el campo, el

\fi124 proceso de adquisicin de la composicin qumica de las aguas en su interaccin
a travs del tiempo
\fi67 con el medio acufero, as como la aplicacin de estos principios para evaluar
el modo en que el agua
\fi3300 adquiere su calidad en los mismos.
\par}{\phpg\posx1136\pvpg\posy4785\absw10919\absh8892 \sl-285 \par\i \f20 \fs21
\cf0 {\b\i0 Palabras}{\b\i0 claves:}{\i0 modelos}{\i0 hidrogeoqumicos,}{\i0 c
intica,}{\i0 acuferos}{\i0 crsicos}{\b\i0 . }
\cf0 \fi4370 {\b ABSTRACT }
\cf0 \fi417 In a previous paper it was dealt with the thermodynamic applications
in hydrogeology, and the
\fi369 thermodynamic fundamentals of the chemical equilibrium were tackled. Its
application was also
\fi60 exemplified in problems related to hydrogeology (Fagundo et al., 2003). I
n this paper the principles of
\fi225 kinetic are discussed, and by means of laboratory and field experiments,
it is shown the acquisition
\fi376 process of the chemical composition of the waters in its interaction thr
oughout the time with the
\fi295 aquifers. Also the application of these principles to assess the way in
which the water acquires its
\fi3518 quality in them is also studied.
\cf0 {\b\i0 Keywords:}{\i0 Hydrogeochemical}{\i0 models,}{\i0 kinetics,}{\i0
karstic}{\i0 aquifers. }
\cf0 {\b\i0 INTRODUCCIN }
{\i0 El}{\i0
modo}{\i0
en}{\i0
que}{\i0
las}{\i0
aguas}{\i0
n
aturales}{\i0
adquieren}{\i0
su}{\i0
composicin}{\i0
est}{\i0
contr
olada}{\i0
por}{\i0
principios }
{\i0 termodinmicos}{\i0
del}{\i0
equilibrio}{\i0
qumico}{\i0
y}{\i0
de}{\i0
la}{\i0
cintica.}{\i0
Al}{\i0
cabo}{\i0
del}{\i0
tiemp
o,}{\i0
en}{\i0
su}{\i0
trayectoria }
{\i0 subterrnea,}{\i0 el}{\i0 control}{\i0 lo}{\i0 ejerce}{\i0 en}{\i0 la}
{\i0 cintica}{\i0 qumica.}{\i0 En}{\i0 muchos}{\i0 trabajos}{\i0 relacionado
s}{\i0 con}{\i0 la}{\i0 calidad }
{\i0 de}{\i0 las}{\i0 aguas}{\i0 naturales,}{\i0 no}{\i0 se}{\i0 consider
a}{\i0 el}{\i0 papel}{\i0 que}{\i0 juega}{\i0 el}{\i0 factor}{\i0 tiempo}
{\i0 en}{\i0 el}{\i0 proceso}{\i0
de}{\i0 disolucin }
{\i0 de}{\i0 los}{\i0 minerales,}{\i0 limitndose}{\i0 solo}{\i0 a}{\i0 e
studiar}{\i0 dicha}{\i0 calidad}{\i0 en}{\i0 condiciones}{\i0 de}{\i0 equi
librio.}{\i0 Sin}{\i0 embargo, }
{\i0 el}{\i0 tiempo}{\i0 de}{\i0 reaccin}{\i0 junto}{\i0 a}{\i0 la}{\i0 t
emperatura}{\i0 y}{\i0 el}{\i0 contenido}{\i0 de}{\i0 CO }{\i0 2}{\i0 ,}{\

i0 son}{\i0 los}{\i0 tres}{\i0 principales}{\i0 elementos }
{\i0 que}{\i0 determinan}{\i0 el}{\i0 proceso}{\i0 de}{\i0 adquisicin}
{\i0 de}{\i0 la}{\i0
composicin}{\i0 qumica}{\i0 a}{\i0 travs}{\i0
e}{\i0 las}{\i0 distintas}{\i0 fases }
{\i0 presentes:}{\i0 gas,}{\i0 lquido}{\i0 y}{\i0 slido.}{\i0 En}{\i0
las}{\i0 condiciones}{\i0 naturales,}{\i0 en}{\i0 un}{\i0 momento}{\i0
dado,}{\i0 el}{\i0 contenido}{\i0 de }
{\i0 CO }{\i0 2}{\i0 libre}{\i0 y}{\i0 de}{\i0 CO }{\i0 2}{\i0 combinado
}{\i0 es}{\i0 el}{\i0 resultado}{\i0 de}{\i0 la}{\i0 accin}{\i0 del}{
\i0 tiempo,}{\i0 as}{\i0 como}{\i0 de}{\i0 las}{\i0 condiciones }
{\i0 geolgicas}{\i0 anteriores}{\i0 (Fagundo,}{\i0 1996). }
{\i0 Para}{\i0 ilustrar}{\i0 el}{\i0 proceso}{\i0 mediante}{\i0 el}{\
i0 cual}{\i0 el}{\i0 agua}{\i0 adquiere}{\i0 su}{\i0 composicin}{\i0
es}{\i0 conveniente}{\i0 realizar }
{\i0 experimentos}{\i0 cinticos}{\i0 en}{\i0 el}{\i0 laboratorio,}{\i0
utilizando}{\i0 minerales}{\i0 solubles}{\i0 tales}{\i0 como}{\i0 hal
ita,}{\i0 yeso}{\i0 o }\par
}
\sect\sectd\pard\plain
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}}\par}{\phpg\posx1623\pvpg\posy1144\absw7615\absh791 \i \f20 \fs18 \cf0 \i \f20
\fs18 \cf0 Contribucin a la Educacin y la Proteccin Ambiental. Vol. 5. (2004) ISBN
959-7136-24-4
\fs14 al. }\par
}
H \par
}
{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \f20 \fs21 \cf0 \f20 \fs21 \cf
0 carbonatos (calcita o dolomita). En el caso de los carbonatos la disolucin, en
presencia de CO {\dn006 \fs14 2} tiene
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-250 \f20 \fs21 \cf0 l
ugar en pocos minutos, no siendo as en el caso de minerales del tipo
aluminosilicato, donde en
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-283 \f20 \fs21 \cf0 c
ondiciones normales, las reacciones alcanzan el equilibrio al cabo de semanas y
aos.
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-325 \f20 \fs21 \cf0 E
l proceso de disolucin de los carbonatos por un agua que contiene un cierto conte
nido de CO {\dn006 \fs14 2} ha sido
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-262 \f20 \fs21 \cf0 e
studiado, desde el punto de vista cintico, por diferentes autores. Entre los trab
ajos publicados a partir
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-283 \f20 \fs21 \cf0 d
e la dcada del 70, se destacan los de Roques y Ek (1973), Berner y Morse (1974),
Sjberg y Rickard
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-283 \f20 \fs21 \cf0 (
1984), Dreybrodt (1992), as como los del colectivo cubano (Fagundo et.
al., 1996; Alvarez et al.,
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-283 \f20 \fs21 \cf0 1
996; Gonzlez et al., 1997).
n este trabajo se presenta un resumen de los resultados experimentales, obtenido
s por el colectivo, con
l objetivo de simular en el de laboratorio los procesos de interaccin
agua roca que ocurren en los
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-283 \f20 \fs21 \cf0 a
cuferos carbonatados.
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-284 \par\f20 \fs21 \c
f0 {\b MATERIALES}{\b Y}{\b MTODOS }
f0 Para la simulacin en el laboratorio de los procesos de interaccin agua - roca
carbonatada se emple
os tipos de reactores:
. Reactor tipo batch de tefln, con una capacidad de 3,5litros, cubier
to con una tapa, tambin de
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-283 \f20 \fs21 \cf0 \
fi360 tefln, con huecos para insertar el agitador, los electrodos y el tubo dispe
rsor del gas. Se realizan
fi360 dos tipos de experimentos: los denominados del tipo REL (se sigue la reacc
in a travs de toma de
fi360 muestras para las determinaciones fsico-qumicas) y los denominados del tipo
CINET (la reaccin
fi360 es seguida a travs de las mediciones directas de los parmetros fsi
co-qumicos (Fagundo et al.,
fi360 1996; Alvarez et al., 1996; Gonzlez, 1997).
. Reactor tipo embudo frita con capacidad de dos litros y porosidad No. 1, por
cuyos poros difunde el

fi360 CO {\dn006 \fs14 2}. Esto permite una mayor difusin del gas al si
stema y una mayor homogeneidad, que se
fi360 produce por el burbujeo del gas en el agua.
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-315 \f20 \fs21 \cf0 L
os experimentos se realizaron de dos formas con respecto al CO {\dn006 \fs14 2}
: en condiciones de sistema abierto
burbujeando el gas todo el tiempo, dejado abierto el manmetro) y en condiciones d
e sistema cerrado
burbujeando un tiempo limitado, cerrando luego el manmetro).
as rocas utilizadas en los experimentos (calizas y dolomas), fueron tam
izadas (80 y 200 mesh) y
aracterizadas por difraccin de rayos X. El CO {\dn006 \fs14 2} utilizado en todo
s los experimentos, fue de un 99,99
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-286 \f20 \fs21 \cf0 %
de pureza envasado en cilindro a una presin de 150 atm (1.5210 Pa).
as mediciones de los diferentes parmetros fsico-qumicos se realizaron con
un pHmetro MPH-4B
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-283 \f20 \fs21 \cf0 C
NIC y un conductmetro ECCA-2 CNIC. Los iones Ca , Mg
y HCO
se determinar
on por mtodos
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-283 \f20 \fs21 \cf0 v
olumtricos, siguiendo las recomendaciones del "{\i Standard}{\i
Meth
ods}{\i
for}{\i
the}{\i
Examination}{\i
of }
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-282 \f20 \fs21 \cf0 {
\i Wastewater}" (APHA; AWWA; WPCF; 1992).
os datos hidroqumicos fueron procesados mediante el sistema informtico SI
MUCIN (Alvarez y
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-283 \f20 \fs21 \cf0 F
agundo, 1995), basado en el modelo cintico experimental.
f0 {\b RESULTADOS}{\b Y}{\b DISCUSIN }
f0 {\b Fundamentos}{\b de}{\b los}{\b experimentos}{\b cinticos}{\b de}{\b
la}{\b disolucin}{\b de}{\b los}{\b carbonatos }
n las investigaciones realizadas en el laboratorio por el colectivo cu
bano (Fagundo et. al., 1996;
\par}{\phpg\posx1135\pvpg\posy2295\absw10812\absh11004 \sl-283 \f20 \fs21 \cf0 A
lvarez et al., 1996; Gonzlez et al., 1997), con el objetivo de esclar
ecer el modo en que las aguas \par
}
\par
}
+
2+ \par
}
{\phpg\posx8199\pvpg\posy11386\absw55\absh160 \f20 \fs14 \cf0 \f20 \fs14 \cf0 \par
}
\par
}
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8a00ffd9
959-7136-24-4
\fs14 al. }\par
}
H \par
}
{\phpg\posx1136\pvpg\posy2295\absw10662\absh599 \f20 \fs21 \cf0 \f20 \fs21 \cf0
naturales adquiere su composicin qumica, se simul el proceso completo de disolucin
de la calcita y
\par}{\phpg\posx1136\pvpg\posy2295\absw10662\absh599 \sl-315 \f20 \fs21 \cf0 la
dolomita, tanto en condiciones de sistema abierto como cerrado con respecto al C
O {\dn006 \fs14 2}: \par
}
{\phpg\posx3939\pvpg\posy2861\absw3900\absh493 \f20 \fs21 \cf0 \f20 \fs21 \cf0 C
O {\dn006 \fs14 2} + H {\dn006 \fs14 2}O + {\ul C}{\ul a}{\ul C}O {\dn006 \fs1
4 3} = Ca
+ 2 HCO{\dn006 \fs14 3 }
\par}{\phpg\posx3939\pvpg\posy2861\absw3900\absh493 \sl-250 \f20 \fs21 \cf0 \fi1
327 Calcita \par
}
CO {\dn006 \fs14 2} + 2 H {\dn006 \fs14 2}O + {\ul C}{\ul a}{\ul M}{\ul g}{\u
l (}{\ul C}O {\dn006 \fs14 3}) {\fs14 2} = Ca{\up006 \fs14 2+ }
876 Dolomita \par
}
{\phpg\posx6533\pvpg\posy2823\absw193\absh160 \f20 \fs14 \cf0 \f20 \fs14 \cf0 2+
\par
}
{\phpg\posx7728\pvpg\posy2823\absw55\absh160 \f20 \fs14 \cf0 \f20 \fs14 \cf0 - \
par
}
{\phpg\posx8026\pvpg\posy2861\absw359\absh239 \f20 \fs21 \cf0 \f20 \fs21 \cf0 (1
) \par
}
{\phpg\posx6927\pvpg\posy3528\absw1962\absh350 \f20 \fs21 \cf0 \f20 \fs21 \cf0 +
Mg {\up006 \fs14 2+} + 4 H CO{\dn006 \fs14 3}{\up006 \fs14 2- }\par
}
) \par
}
{\phpg\posx1136\pvpg\posy4155\absw8876\absh239 \f20 \fs21 \cf0 \f20 \fs21 \cf0 E
ste proceso puede ser expresado mediante una ecuacin cintica deducida a partir de
: \par
}
{\phpg\posx1188\pvpg\posy4438\absw333\absh547 \f20 \fs21 \cf0 \f20 \fs21 \cf0 dC
dt \par
}
{\phpg\posx1169\pvpg\posy5072\absw146\absh239 \f20 \fs21 \cf0 \f20 \fs21 \cf0 c
\par
}
{\phpg\posx1277\pvpg\posy5209\absw281\absh239 \f20 \fs21 \cf0 \f20 \fs21 \cf0 eq
\par
}
{\phpg\posx1553\pvpg\posy4564\absw733\absh281 \f40 \fs21 \cf0 \f40 \fs21 \cf0 ={
\f20 k}{\f20 (C }\par
}
{\phpg\posx1577\pvpg\posy5072\absw91\absh239 \f20 \fs21 \cf0 \f20 \fs21 \cf0 : \
par
}
{\phpg\posx2208\pvpg\posy4729\absw281\absh239 \f20 \fs21 \cf0 \f20 \fs21 \cf0 eq
\par
}
{\phpg\posx2504\pvpg\posy4564\absw488\absh281 \f40 \fs21 \cf0 \f40 \fs21 \cf0 {\
field{\*\fldinst SYMBOL 45 \\f Symbol }}{\f20 C) }\par
}
{\phpg\posx3195\pvpg\posy4592\absw1194\absh239 \f20 \fs21 \cf0 \f20 \fs21 \cf0 (
3), donde: \par
}
{\phpg\posx5028\pvpg\posy4592\absw6375\absh239 \f20 \fs21 \cf0 \f20 \fs21 \cf0 e
s la velocidad de reaccin; k: la constante de velocidad; \par
}
{\phpg\posx1916\pvpg\posy5072\absw9707\absh331 \f20 \fs21 \cf0 \f20 \fs21 \cf0 l
as concentraciones de Ca , Mg (calizas dolomitizadas y dolomitas), y HCO {\
dn006 \fs14 3} en el equilibrio \par
}
{\phpg\posx4385\pvpg\posy4438\absw448\absh695 \f20 \fs21 \cf0 \fi115 \f20 \fs21
\cf0 dC
6 dt
\par}{\phpg\posx4385\pvpg\posy4438\absw448\absh695 \sl-181 \f20 \fs21 \cf0 {\fs1
4 2+ }\par
}
{\phpg\posx5072\pvpg\posy5033\absw193\absh160 \f20 \fs14 \cf0 \f20 \fs14 \cf0 2+
\par
}
{\phpg\posx9538\pvpg\posy5033\absw55\absh160 \f20 \fs14 \cf0 \f20 \fs14 \cf0 - \
par
}
qumico; y C es la concentracin de esos iones en el tiempo t. Despejando C e integr
ando la expresin
\par}{\phpg\posx1135\pvpg\posy5537\absw10605\absh493 \sl-283 \f20 \fs21 \cf0 (3)
, se obtiene la ecuacin que expresa la variacin de la concentracin inica en el tiemp
o (Fig. 1): \par
}
{\phpg\posx5057\pvpg\posy6164\absw918\absh293 \f20 \fs21 \cf0 \f20 \fs21 \cf0 C
= Ceq \par
}
-{\dn006 -kte }\par
}
{\phpg\posx6708\pvpg\posy6164\absw580\absh239 \f20 \fs21 \cf0 \f20 \fs21 \cf0 )
(4) \par
}
Figura 1: Variacin en el tiempo de las concentraciones de CO 2, HCO 3 , Ca \par
}
{\phpg\posx8206\pvpg\posy11585\absw110\absh239 \f20 \fs21 \cf0 \f20 \fs21 \cf0 \par
}
2+ y Mg2+ \par
}
, del pH y la \par
}
{\phpg\posx1135\pvpg\posy11989\absw10666\absh748 \f20 \fs21 \cf0 \fi2887 \f20 \f
s21 \cf0 conductividad elctrica del fichero Cinet17.
\par}{\phpg\posx1135\pvpg\posy11989\absw10666\absh748 \sl-283 \f20 \fs21 \cf0 En
los trabajos de simulacin del proceso de interaccin agua-roca en el laboratorio,
en las condiciones
\par}{\phpg\posx1135\pvpg\posy11989\absw10666\absh748 \sl-283 \f20 \fs21 \cf0 ex
perimentales realizadas, qued demostrado que esta expresin es en realidad de pseud
o primer orden \par
}
(Fagundo, 1996; Alvarez et al, 1996): \par
}
C{\dn006 \fs17 =} Ceq{\fs17 (1}{\fs17 -}{\fs25 e}-kt \par
}
{\phpg\posx6567\pvpg\posy13083\absw110\absh179 \f20 \fs16 \cf0 \f20 \fs16 \cf0 n
\par
}
{\phpg\posx6704\pvpg\posy13256\absw73\absh198 \f20 \fs17 \cf0 \f20 \fs17 \cf0 )
\par
}
{\phpg\posx7073\pvpg\posy13217\absw530\absh239 \f20 \fs21 \cf0 \f20 \fs21 \cf0 (
4 a) \par
}
donde n, es un coeficiente experimental que toma valores entre 0 y 1 (Fig. 2). \
par
}
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d9
959-7136-24-4
\fs14 al. }\par
}
H \par
}
Figura 2: Resultados comparativos entre los valores reales y los obte
nidos por simulacin para el fichero Cinet17, con
\par}{\phpg\posx1135\pvpg\posy7373\absw10772\absh3479 \sl-235 \f20 \fs18 \cf0 n=
0.67
\par}{\phpg\posx1135\pvpg\posy7373\absw10772\absh3479 \sl-271 \f20 \fs18 \cf0 {\
fs21 En}{\fs21 la}{\fs21 figura}{\fs21 3}{\fs21 se}{\fs21 ilustra,}{\f
s21 mediante}{\fs21 el}{\fs21 diagrama}{\fs21 de}{\fs21 Tillman}{\fs21
Trombe,}{\fs21
el}{\fs21
comportamiento}{\fs21
de}{\fs21 un }
fs21 experimento}{\fs21 de}{\fs21 interaccin}{\fs21 agua}{\fs21 -}{\fs21 roc
a}{\fs21 carbonatada,}{\fs21 cuya}{\fs21 tendencia}{\fs21 es}{\fs21 alcanza
r}{\fs21 el}{\fs21 equilibrio}{\fs21 al}{\fs21 final}{\fs21 de }
fs21 la}{\fs21 reaccin.}{\fs21 En}{\fs21 dependencia}{\fs21 del}{\fs21 conte
nido}{\fs21 de}{\fs21 CO }{\dn006 \fs14 2}{\fs21 disponible,}{\fs21 el}{\f
s21 agua}{\fs21 adquiere}{\fs21 en}{\fs21 el}{\fs21 mismo}{\fs21 mayor}{\f
s21 o }
fs21 menor}{\fs21 dureza. }
b \fs21 Evaluacin}{\b \fs21 del}{\b \fs21 efecto}{\b \fs21 de}{\b \fs21 l
os}{\b \fs21 factores}{\b \fs21 que}{\b \fs21 controlan}{\b \fs21 la}{\b
\fs21 disolucin}{\b \fs21 de}{\b \fs21 los}{\b \fs21 carbonatos}{\b \fs2
1 mediante }
b \fs21 experimentos}{\b \fs21 cinticos }
fs21 Con}{\fs21 el}{\fs21 objetivo}{\fs21 de}{\fs21 evaluar}{\fs21 el}
{\fs21 papel}{\fs21 que}{\fs21 ejercen}{\fs21 los}{\fs21 diferentes}{\
fs21 factores}{\fs21 que}{\fs21 determinan}{\fs21 la}{\fs21 cintica}{\f
s21 de }
fs21 disolucin}{\fs21 de}{\fs21 los}{\fs21 carbonatos}{\fs21 (temperatura,}{\
fs21 velocidad}{\fs21 de}{\fs21 agitacin,}{\fs21 contenido}{\fs21 y}{\fs21
forma}{\fs21 de}{\fs21 suministro}{\fs21 del }
fs21 CO }{\dn006 \fs14 2}{\fs21 ,}{\fs21 cantidad}{\fs21 disponible}{\fs21 y
}{\fs21 tipo}{\fs21 de}{\fs21 roca),}{\fs21 ser}{\fs21 realizaron}{\fs21
varios}{\fs21 experimentos}{\fs21 cinticos}{\fs21 (Tabla}{\fs21 1).}{\fs21 C
omo }
fs21 indicador}{\fs21 de}{\fs21 eficiencia}{\fs21 del}{\fs21 proceso,}{\fs21
se}{\fs21 tom}{\fs21 el}{\fs21 incremento}{\fs21 de}{\fs21 dureza}{\fs21
en}{\fs21 el}{\fs21 agua}{\fs21 del}{\fs21 reactor}{\fs21 al}{\fs21 fina
l}{\fs21 de }
fs21 la}{\fs21 reaccin}{\fs21 (}{\f40 \fs21 {\f63 \u8710\'3f}}{\fs21 CaCO }{\dn
006 \fs14 3}{\fs21 ),}{\fs21 el}{\fs21 cual}{\fs21 es}{\fs21 proporcional}{
\fs21 a}{\fs21 la}{\fs21 diferencia}{\fs21 de}{\fs21 conductividad}{\fs21
elctrica}{\fs21 final}{\fs21 (CE }{\dn006 \fs14 f}{\fs21 ).}{\fs21 Los }
fs21 resultados}{\fs21 fueron}{\fs21 los}{\fs21 siguientes: }\par
}
. \par
}
{\phpg\posx1495\pvpg\posy11257\absw10244\absh3075 \f20 \fs21 \cf0 \f20 \fs21 \cf
0 Aunque de poca magnitud, se apreci como tendencia, un mayor contenido
de la dureza al
isminuir la temperatura. En los experimentos CINET 2 y 16, realizados a diferent
es temperaturas
n condiciones similares, se aprecia una disminucin de 128 mg/L de CaCO {\dn006 \f
s14 3} disuelto al aumentar 3
fi79 C la temperatura del agua. Este efecto, que est regido por la ley de Arheniu
s, es ms significativo
las aguas termales procedente del drenaje profundo de los acuferos.
a dureza del agua al final de la reaccin es mucho mayor cuando la de la velocidad
de agitacin es
\par}{\phpg\posx1495\pvpg\posy11257\absw10244\absh3075 \sl-315 \f20 \fs21 \cf0 m
ayor debido a que se garantiza una mejor difusin del CO {\dn006 \fs14
2} (experimentos CINET 6 y 12
\par}{\phpg\posx1495\pvpg\posy11257\absw10244\absh3075 \sl-250 \f20 \fs21 \cf0 r

ealizados con velocidades de 500 y 0 rpm respectivamente, manteniendo
en forma similar los
\par}{\phpg\posx1495\pvpg\posy11257\absw10244\absh3075 \sl-315 \f20 \fs21 \cf0 r
estantes parmetros). Con una agitacin de 500 rpm se alcanza 200 mg/l ms de CaCO {
\dn006 \fs14 3} disuelto
\par}{\phpg\posx1495\pvpg\posy11257\absw10244\absh3075 \sl-250 \f20 \fs21 \cf0 q
ue sin agitacin.
as mayores concentraciones de carbonato de calcio disuelto se obtienen
utilizando mayores
ontenidos de CO {\dn006 \fs14 2} (experimentos CINET 2, 16, 6 y 12). \par
}
{\phpg\posx1496\pvpg\posy12067\absw91\absh160 \f20 \fs14 \cf0 \f20 \fs14 \cf0 o
\par
}
. \par
}
. \par
}
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959-7136-24-4
\fs14 al. }\par
}
H \par
}
{\phpg\posx1136\pvpg\posy2333\absw158\absh198 \f20 \fs18 \cf0 \f20 \fs18 \cf0 4.
\par
}
{\phpg\posx1136\pvpg\posy3183\absw158\absh708 \f20 \fs18 \cf0 \f20 \fs18 \cf0 5.
\par}{\phpg\posx1136\pvpg\posy3183\absw158\absh708 \sl-283 \par\f20 \fs18 \cf0 6
. \par
}
La dureza que adquiere el agua se incrementa a medida que la cantid
ad de roca disponible en el
\par}{\phpg\posx1496\pvpg\posy2295\absw10249\absh1768 \sl-315 \f20 \fs21 \cf0 re
actor es mayor, tanto en condiciones de sistema abierto como
cerrado respecto al CO{\dn006 \fs14 2 }
\par}{\phpg\posx1496\pvpg\posy2295\absw10249\absh1768 \sl-250 \f20 \fs21 \cf0 (e
xperimentos CINET 2 y 14, y CINET 3 y 18 respectivamente).
\par}{\phpg\posx1496\pvpg\posy2295\absw10249\absh1768 \sl-283 \f20 \fs21 \cf0 La
s calizas son ms solubles que las dolomas en las condiciones estudiadas (experime
ntos CINET
y 7).
\par}{\phpg\posx1496\pvpg\posy2295\absw10249\absh1768 \sl-283 \f20 \fs21 \cf0 La
composicin qumica de las aguas resultantes de los experimentos cinticos es simil
ar a las de
\par}{\phpg\posx1496\pvpg\posy2295\absw10249\absh1768 \sl-283 \f20 \fs21 \cf0 lo
s acuferos crsicos (aguas bicarbonatadas clcicas). \par
}
{\phpg\posx1136\pvpg\posy10501\absw10830\absh3338 \f20 \fs21 \cf0 \fi148 \f20 \f
s21 \cf0 Figura 3. Diagrama de Tillaman Trombe donde se aprecia la variacin de la
concentracin de CaCO{\dn006 \fs14 3 }
fi1444 hasta el establecimiento del equilibrio qumico (experimento CINET18).
as magnitudes de pCO{\dn006 \fs14 2}
se expresan en atmsferas con el
objetivo de que resultados puedan
ompararse con reportados por otros investigadores, ya que en la litera
tura especializada se utiliza
fi9883 {\fs16 5 }
ichas unidades. Para cualquier otra consideracin se debe tener en cuenta que 1
atm. = 1.01325 10
\par}{\phpg\posx1136\pvpg\posy10501\absw10830\absh3338 \sl-292 \f20 \fs21 \cf0 P
a.
f0 {\b Concentraciones}{\b de}{\b carbonato}{\b de}{\b calcio}{\b en}{\b a
cuferos}{\b crsicos,}{\b comparacin}{\b con}{\b los}{\b resultados}{\b de }
\par}{\phpg\posx1136\pvpg\posy10501\absw10830\absh3338 \sl-283 \f20 \fs21 \cf0 {
\b los}{\b experimentos}{\b cinticos }
f0 En la tabla 2 se muestran las concentraciones en mg/L de CaCO {\dn006 \fs14
3} disuelto de algunas fuentes crsicas
pozos y manantiales) en el pas, con el objetivo de comparar sus magnitudes con la
s alcanzadas en los
xperimentos cinticos que aparece en la tabla 1. \par
}
}

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