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Abstract
One of the greatest challenges of the 21st Century is to develop a method for remediating
high level nuclear waste generated by fission-based power production systems. In the
wake of the Fukushima catastrophe, the sense of urgency driving this initiative has never
been greater. The problems associated with reducing alpha, gamma and beta emissions
generated by high level solid and liquid nuclear waste materials are technically difficult
for a variety of reasons. The purpose of this project is to suggest alternative approaches
which can be designed, tested, prototyped and adapted to satisfy the technical, scientific,
and engineering problems associated with reducing radioactive emissions generated by
spent nuclear fuel waste materials to ambient background levels. (Exhibit A Methods
for Neutralizing Radioactivity)
The remediation techniques described here have been shown to be effective in the
treatment of various kinds of nuclear waste materials. The preferred technique exploits
the nature of a patented phenomenological process referred to in the literature as High
Density Charge Clusters [HDCC] to temporarily disaggregate the nuclear structure of
target materials, thereby inducing lower energy states and thereby shortening the half-life
of the daughter products of nuclear decay. The product of the HDCC process is a
reduction in the intensity, rate of emissions, and half-life of target materials by up to
50.00% with each interaction. (Exhibit C Mathematical Model)
A multi-phased approach is proposed to resolve the scientific, engineering and technical
problems related to the development of a suitable methodology in five successive
research, design & development phases. Estimated cost to complete the first three phases
which will deliver field testable beta units in six fields of application is less than
$10,000,000.00. Each phase is estimated to require between 12 18 months, with a total
expected project term of 3 5 years. (Exhibit B Phased Development Schedule and
Budget)
Background
More than 30 techniques for mitigating radioactive emissions in spent nuclear fuel waste
materials have been proposed and experimentally tested over the past 50 years. A partial
list of alternatives is attached as Exhibit A Methods For Neutralizing Radioactivity.
They range from simple incineration of low level waste in a 7000F furnace to
catastrophic destruction of the elemental materials via a process called nuclear spallation.
waste,
contaminated environmental media,
surplus facilities, and
materials in inventory.
This proposal focuses on the first two components. Nuclear weapons production in the
United States is comprised of a complex series of manufacturing operations, each of
which generates large quantities of nuclear and chemical wastes. The term waste is
defined as solids or liquids that are radioactive, chemically hazardous, or both. This waste
consists of materials that have been disposed of previously, await disposal, or have been
retrieved in site cleanups and are currently in storage. Waste is measured in terms of
volume (cubic meters) and radioactivity (curies). Waste from nuclear weapons production
managed by DOE includes 24 million cubic meters containing 900 million curies.
The major categories of waste are:
high-level waste,
transuranic waste,
low-level waste,
mixed low-level waste,
11e(2) byproduct material,
hazardous waste, and
THER waste.
High-level waste is the highly radioactive waste resulting from spent nuclear fuel
generated by power production or power reactors, as well as from the chemical
processing of spent nuclear fuel and irradiated target assemblies. The radioactivity comes
from fission fragments and their daughter products resulting from the fission of U-235 in
production reactors. Although radiation from short-lived fission products (fragments and
their daughters) will decrease dramatically in the next hundred years, radiation risks
associated with the long-lived products already on and will remain high for thousands of
years. In the initial decay period, most of the radioactivity is due to Cs-137, Sr-90, and
their short-lived daughter products. Plutonium, americium, uranium, and their daughter
products are the major contributors to long-term radioactivity.
Transuranic
(TRU)
waste
contains
alpha-emitting
transuranic
elements
or
actinides with half-lives of greater than 20 years and a combined activity of greater than
100 nanocuries per gram of waste. Because of the long half-lives of many TRU isotopes,
TRU waste can remain radioactive for hundreds of thousands of years. Some common
isotopes found in TRU are Pu-238, Pu-239, Pu-240, Pu-241, Pu-242, Am-241, and Cu244. TRU waste results from the fabrication of plutonium components, recycling of
plutonium from scrap, retired weapons, and chemical separation of plutonium. Unlike
high-level waste, which results from a few specific processes with a narrow range of
physical matrices and chemical characteristics, TRU waste exists in many forms with a
spectrum of chemical properties.
A small percentage of TRU waste exhibits high direct exposure hazards and is referred to
as "remote-handled" TRU waste. The majority of TRU waste emits low levels of direct
radiation and is called "contact-handled" waste. The chief hazard of "contact-handled"
waste is due to alpha radiation. Alpha particles cannot penetrate the skin but cause serious
localized tissue damage when inhaled or ingested. When inhaled, TRU elements tend to
accumulate in the lungs; soluble TRU compounds migrate through the body,
accumulating in the bone marrow and liver.
Unanswered Questions
Among the questions that must be addressed, the following are of primary importance:
1. Variable Treatment Requirements for Liquid waste v. solid waste [statistical
assessment in gallons, tons, approaches, methodologies, technological alternatives
etc.]
2. Calculations nuclear bonding energies. What is the threshold energy required to
temporarily disrupt the integrity of the targeted nucleus?
3. Modeling Requirements - Schematic diagrams, animated illustration of nuclear
structures in action, individually and adjacent to other materials in a crystalline
lattice
4. Calculations SED [stochastic electrodynamic] model of radioactive decay [i.e.,
how many decay stages are needed to reduce current emission structure to
generate ambient background levels of gamma, alpha & beta emissions]
5. Calculations When minimal disaggregation energy is applied, how much energy
is released over what t? What form does the output energy take? What is
required to manage it?
6. Calculations When temporary disaggregation occurs, how long before
reformation occurs, and in what form(s)? What effect does this dynamic exert on
half-life and rate of radioactive emissions & decay cycles? Proposed
Methodology
Proposed Approach
Liquefied Radioactive Waste
Most treatment and conditioning processes for Low and Intermediate Level Waste
[LILW] have now reached an advanced industrial scale. Although these processes and
technologies are sufficient for effective management of radioactive waste at nuclear
power plants, further improvements in this technology are still possible and desirable.
The increasing cost of radioactive waste disposal provides an incentive to adopt
procedures and techniques to minimize waste quantities and to develop new techniques to
minimize volumes at the treatment and conditioning step.
Some examples of such new developments include the use of specific inorganic sorbents
to improve liquid waste treatment; use of membrane techniques for liquid waste
treatment; de-watering and drying of bead resin and filters slurries; incineration of spent
ion-exchange resins; dry cleaning of protective cloth to reduce quantity of laundry drains;
use of high integrity containers for packaged dried filter sludges; vitrification of some
intermediate-level waste to reduce volumes of waste to be disposed of; and supercompaction of unburnable waste.
HDCCs exhibit a tendency to link up like beads in a chain. The spacing of the beads in
the chain is approximately equal to the diameter of the individual beads. The HDCC
chains have been observed to form closed ring-like structures as large as 20 microns in
4
5
6
7
Shoulders Patents
Mesyats Patent
Jin mathematical formulations
Jin, S-X, EVO plasma discharge toroidal structure image, ref.
The toroidal form of the EVO has been photographed with high resolution tunneling
electron microscopes at the point of emission. This phenomenon, which demonstrates the
dynamics of self-organizing criticality and super-symmetry at subatomic scales, is
specifically prohibited by the standard model of physics because it is believed to violate
the Pauli Exclusion Principle. Nevertheless, as the photographic and digital imaging
evidence shows, the toroid formed by the self-organizing behavior of the electrons in a
vacuum/plasma is both stable and can be directed through a proton-rich environment
along the flux lines of properly aligned magnetic fields, to collide with a target material.
Figure 10
8
This image was produced by T. Banchoff and his colleagues at the University of
Illinois, in concert with N. Thompson at Brown University and D. Banks of the
University of North Carolina and Langley Research Center. It is of no small interest to
the authors that this figure was produced with Y-Bias and Angularity data as an
expression of a topological model.
in 3-Sphere [9]
Coming from the EVO source at the lower portion of the pinhole
camera image, the EVO is seen to follow a helical pattern of motion,
sequentially decomposing into individual electrons as it moves at a
rate of 1/10 the velocity of light to the top of the photo. The length of
9
http://www.geom.uiuc.edu/docs/research/ieee94/node25.html
The ability to penetrate is tied to having an electrical impedance match for the EVO
upon emergence into the space beyond the foil. Deep penetration of the materials
depends upon having a form of impedance match between the foil and the airspace.
10
View of Dual
Vacuum
Figure 13
Schematic Diagram of HDCC Accelerator
Radioactivity Remediation System
11
ttp://www.svn.net/krscfs/Electromagnetic%20Pulse%20Source%20Using
%20Fluidized%20Electrons-Appendix%20I.PDF
HDCC trajectories
Anode
Cathode
Accelerated
ring
Electron
beem
After compression
and ion loading
Instead, at the point of impact, light [in the form of highly energized photons], heat [in
the form of infrared emissions], gamma rays and neutrons are emitted as the result of the
disaggregating effect of the collision. Within narrow limits, during the femto-seconds
following the impact event, the hadrons disaggregated to form a plasma automatically rearrange themselves to create a nuclear structure which demonstrates a quantum reduction
of energy, to constitute what is referred to as a more 'steady state,' that is, a condition in
which the number and volume of neutrons, gamma rays and other products of nuclear
decay are reduced to a lower energy state. This process results in a shortening of the halflife of the target material by 50.0% with each collision and reorganizing event.
Figure 18 shows that a significant quantity of atomically modified material is found in the
residue created during the bombardment of 232Thorium by HDCCs during Jins test
protocols. 232Protactinium is a daughter product generated by 232Thorium during its
normal beta-decay cycle. The implications arising from this scientifically validated
protocol are quite profound. The procedures developed by Jin et al demonstrate that a low
voltage power source can be harnessed to drive a properly engineered electron emitting
apparatus in a way that results in the reduction of gamma, neutron and photon emissions
in a target material, without the danger of triggering any sort of catastrophic fission event.
The research also strongly suggests that this apparatus can be design-engineered to
12
Jin used a Ludlum Measurements, Inc., Sodium Iodide detector, Model 4410-D; the
Aptec Autobias PC Card, Aptec Multi-channel analyzer [Series 5000 MCard], and
Aptect Basic Display and Acquisition Software [PCMCA/SUPER]. This combination
provides a relatively low-cost gamma-ray spectroscope.
References
1. H. Alfven and P. Wernholm, Arkiv Fysik 5, 175 (1952).
2. C. Joshi, et al., Nature, Vol. 311, No. 5986, 525 (1984).
3. C. L. Olson, Report SLA-73-0865, Sandia Laboratories (1974).
4. M. L. Sloan and W. E. Drummond, Phys. Rev. Lett. 31, 1234 (1973).
5. P. Sporangial, et al., Phys. Rev. Lett. 36, 1180 (1976).
6. G. I. Budker, Proc. CERN Symposium on High energy Accelerators and Pion Physics, Geneva,
Vol. 1 (1956).
7. C. L. Olson, et al., Phys. Rev. Lett. 56, 2260 (1986)
8. Kenneth R. Shoulders, "Method of and Apparatus for Production and Manipulations of High
Density Charge", U.S. Patent 5,054,046, issued Oct 1, 1991.
9. Kenneth R. Shoulders, "Circuits Responsive to and Controlling Charged Particles", U.S. Patent
5,054,047, issued Oct 1, 1991.
10. Kenneth R. Shoulders, "Energy Conversion Using High Charge Density," U.S. Patent
5,018,180, issued May 21, 1991.
11. Kenneth R. Shoulders, EV, A Tale of Discovery, c1987, published and available from the
author, P.O. Box 243, Bodega, CA 94922-0243.
12. G.A. Mesyats, "Ecton Processes at the Cathode in a Vacuum Discharge", Proceedings of the
XVIIth international Symposium on Discharges and Electrical Insulation in Vacuum, July 21_26,
1996, Berkeley, Calif., pp 720-731, 38 refs, 10 figs, 5 tables.
13. Shang Xian Jin & Hal Fox, "Characteristics of High Density Charge Clusters: A Theoretical
Model",
J. of New Energy, vol. 1, no 4, Winter 1996, pp 5-20, 16 refs, 2 figs.
14. Ken Shoulders & Steve Shoulders, "Observations on the Role of Charge Clusters in Nuclear
Cluster Reactions", J. of New Energy, vol. 1, no 3, pp 111-121, Fall 1996, 7 refs, 22 figs.
3.
4. R&D various collective ion acceleration concept, and select best acceleration scheme
Electron ring acceleration
Neutral gas-filled drift tube
PROPRIETARY & CONFIDENTIAL
For Internal Management Use Only Not For Unauthorized Disclosure
Page 27
EXHIBIT C
[] Mathematical Model
Jin, Shoulders & Yurth have provided the following formulation for estimating the maximum electric
field and holding power in a HDCC ring. As an approximation of the HDCC ring, consider an electron
ring with major radius R, minor radius a, and uniform electron density ne, in a background of ions
(charge +Ze) of uniform density ni. If we assume a/R << 1, then the self-electric field Er of the
slender ring could be expressed approximately in cylindrical coordinates (r, , z) by (in MKSA units)
Em = ener/20 (1 fe)
(1)
where fe = Z ne/ni is a charge neutralization factor. The maximum electric field in the ring could be
estimated by the electric field at the edge of the ring ( r = a): Em = enea/20 (1 fe), or using the
total number of electrons in the ring, Ne = 22a2R ne, it can be written as
Em = Ne/420aR (1 fe)
(2)
(V/m)
(3)
In order for the ions to be accelerated along with the electron ring, the ions must be held within the ring
during the acceleration. The holding power is defined as the maximum electric field holding the ions
in the accelerated ring, Eh . The Eh is related to the maximum electric field Em and can be expressed as
Eh = Em
(4)
Because of the neutralization effect of the ions, the Eh is always smaller than Em, i.e. < 1. The size
depends on the ion number and distribution in the electron ring. As an example, consider the 20
m diameter HDCC ring. With the data given by Ken Shoulders, we have a ~ 0.5 m , R ~ 10 m,
Ne ~ 1013 and fe ~105<< 1, and therefore, we get Em ~ 1014 V/m, and
of
Eh 1014 V/m
(5)
This field strength calculation shows that the collective electric field in the HDCC ring is millions of
times stronger than the electric field in a normally intense relativistic electron beam ( ~100 MV/m), or
about eight orders of magnitude increase compared with the average electric field limit in conventional
accelerators (1 - 5 MV/m). This holding power is therefore strong enough to hold ions in the moving
potential well of the ring during the acceleration.
There is a possibility that using a specially designed multi-tip cathode array and a properly calibrated
magnetic field [as shown in Figure 13], a large high density electron ring with dimensions much larger
than the 20 microns could be generated. For example, consider a situation in which a large amount of
HDCC produced by a cathode, such as a metal-dielectric cathode, could be injected into a cusped
magnetic field. The magnetic field would be designed to transform the initially longitudinally oriented
electron velocity into an azimuthally oriented velocity. With this strategy, the HDCC beam could be
accumulated into a large high-density electron ring. The holding power of the electron ring would be
strong enough to hold large amount of ions (e.g., protons) and the ions could be collectively accelerated
to a high energies.
Consider the ion loaded electron ring with sufficiently high holding power in an external axial (z)
electric field E. The rate of energy gain of the ion energy Wi in the axial direction is then
(6)
where Mi and me are the ion and electron rest mass, fe = Zni/ne is a charge neutralization factor, ni and
ne are the ion and electron number, Z is the charge state of the ion, vc = (1 (ve/c)2 )1/2 is the
relativistic factor, ve is speed of the electron cluster, and c is speed of light. In the case of small ion
loading comparing with electron number, i.e. fe = Zni /ne << Zc me/Mi , Eq. (6) reduces to
(7)
(8)
where V is the applied potential difference and We is the electron kinetic energy. In the same potential
difference V, the energy gain of a pure ion is
Wi = ZeV
(9)
(10)
where A is atomic weight of the ion. This means that the ion acceleration induced by an electron cluster
is about 1836 A/Z times more effective than pure ion acceleration. Table 1 shows some applied
potential differences and the kinetic energy of a proton (deuteron) collectively accelerated by the
electron cluster.
As an example, consider a neutron-producing reaction:
Li7
Be7 + n,
In this reaction the proton energy must be not less than the reaction threshold of 1.88 MeV. To achieve
this proton energy in a conventional accelerator, the applied total electric potential differences must be
not less than 1.88 MV. In the high density charge cluster accelerator, however, the required potential
differences for the same proton energy is only 1.88 MV/1836 = 1.02 KV.