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journal homepage: www.elsevier.com/locate/atmosenv
The effect of SRTM and Corine Land Cover data on calculated gas and
PM10 concentrations in WRF-Chem
A. De Meij a, *, E. Bossioli b, C. Penard a, J.F. Vinuesa a, I. Price a
a
b
h i g h l i g h t s
Differences are found in the land cover classes between Corine and USGS data sets.
T2 and winds are different between WRF-Chem with SRTM Corine LC and with USGS.
SH, LH and PBLs are different between WRF-Chem with SRTM Corine LC and USGS.
WRF-Chem with SRTM Corine LC calculates higher gas concentrations than with USGS.
WRF-Chem with SRTM Corine LC calculates higher PM10 concentrations than with USGS.
a r t i c l e i n f o
a b s t r a c t
Article history:
Received 29 July 2014
Received in revised form
12 November 2014
Accepted 14 November 2014
Available online 15 November 2014
The goal of this study is to investigate the impact of the high resolution Shuttle Radar Topography
Mission (SRTM) 90 m 90 m topography data, together with the 100 m 100 m resolution Corine Land
Cover 2006 on the simulated gas and particulate matter (PM10) concentrations by WRF-Chem. We
focused our analysis on the well-known highly urbanized region of the Po Valley. Large differences are
found in the geographical distribution of the land cover classes between Corine Land Cover and 30 arc
seconds USGS. The simulation with the SRTM and Corine Land Cover increases modelled temperature at
2 m and reduces wind speeds due to more friction at the surface induced by the Corine Land Cover.
Latent and sensible heat uxes show large differences between the two simulations and the related
boundary layer development and depth. The simulation with the SRTM and Corine Land Cover favours
the precipitation amount over a large of part the Alps and follows the pattern of the difference in
topography between the two topography data sets. In term of air quality indicators, impacts are also large
and geographical dependent. Monthly average of CO, NO and SO2 concentrations over a large part of the
Po Valley are higher when using Corine Land Cover, up to ~20, ~50 and ~55%, respectively. With respect
to PM10, the impacts are also geographical dependent. Over the Po valley area, calculated PM10 concentrations are in general higher using Corine Land Cover (up to 6.7 ug/m3 [~26%] westerly of Milan)
while differences are smaller over the Alps (~0.25ug/m3 [~20%]). Although the scope of this work is not to
evaluate the model performance in calculated meteorological parameters and gas and PM10 concentrations, calculated values by the simulation with SRTM and Corine Land Cover show a better agreement
with the observations than the simulation with the USGS topography and land cover data sets. A
quantitative comparison between modelled and observed monthly average PM10 concentrations shows
that both simulations underestimate the observed PM10 concentrations by a factor ~4. The agreement is
much better during episodes for the simulation with the SRTM and Corine Land Cover. For CO, SO2 and
NOx, the modelled monthly mean concentrations are similar for the two simulations. Larger differences
are found during some episodes and regions with the SRTM and Corine LC simulation being in better
agreement with the observations.
2014 Elsevier Ltd. All rights reserved.
Keywords:
WRF-Chem
Corine Land Cover
SRTM
USGS Land Cover
* Corresponding author.
E-mail address: alexander.demeij@noveltis.fr (A. De Meij).
http://dx.doi.org/10.1016/j.atmosenv.2014.11.033
1352-2310/ 2014 Elsevier Ltd. All rights reserved.
178
1. Introduction
A common problem in air quality modelling is the underestimation of simulated particulate matter (PM) concentrations by air
chemistry transport models (ACTMs). Many model studies (Tsyro,
2003; De Meij et al., 2007; Vautard et al., 2007; Stern et al., 2008;
De Meij et al., 2008; De Meij et al., 2009; Vautard et al., 2009),
and coordinated modelling activities such as Citydelta [http://aqm.
jrc.ec.europa.eu/citydelta/], AEROCOM [http://aerocom.met.no/
aerocomhome.html] and Eurodelta [http://aqm.jrc.ec.europa.eu/
eurodelta/] showed that ACTMs in general underestimate
observed PM concentrations over Europe. The City Delta exercise
(http://aqm.jrc.ec.europa.eu/citydelta/, Cuvelier et al., 2006; Thunis
et al., 2007; Vautard et al., 2006) showed that simulated PM concentrations are underestimated by the ACTMs for Milan (Italy),
especially for winter time episodes. There are several reasons for
the underestimation of PM10 e.g. unaccounted sources of emissions, vertical and temporal distribution of the emissions and that
the Po Valley is characterized by very low wind speeds and frequent
weak circulation conditions. These stagnant meteorological conditions are difcult to simulate by prognostic and diagnostic
models over complex areas (Dosio et al., 2002; Minguzzi et al.,
2005; Carvalho et al., 2006; Stern et al., 2008; De Meij et al.,
2009; Ritter et al., 2013), which contribute to the underestimation of simulated PM concentrations.
Aerosol formation processes are known to be non-linear
dependent on gas concentrations (West et al., 1998) and meteorological variables (Haywood and Ramaswamy, 1998). Recent studies
have shown the impact of meteorological parameters on gas and
aerosol calculated concentrations by altering, for example the
planetary boundary layer scheme, micro-physics scheme, land
surface physic schemes (De Meij et al., 2009; Appel et al., 2010;
Zabkar
et al., 2013; Forkel et al., 2014).
A recent study by De Meij and Vinuesa (2014) showed the
impact of the high resolution (100 100 m) Corine Land Cover on
calculated meteorological parameters (wind speed, temperature
and precipitation) during a winter and a summer period, by
comparing with a simulation using the standard 30-arc seconds
(~1 1 km) USGS Land Cover and observations. They found large
differences in the fraction of urban built-up area between the
Corine Land Cover and USGS Land Cover for the Lombardi province
(Italy), which impacted the calculated meteorological parameters.
The simulation with the Corine Land Cover resulted in lower wind
speeds and showed a better agreement with the observations. The
accuracy of land-use classications in meteorological modelling
affects some of the meteorological parameters. Urban built-up
areas are more likely to trap solar radiation and reduce wind
speeds than open rural areas, which may impact the temperatures,
buoyancy and wind directions and wind speeds. A good estimate of
meteorological variables such as wind speed is therefore crucial for
calculating gas and aerosol impacts on air quality and climate
change, and evaluating coherent reduction strategies.
To our knowledge the impact of topography and Corine Land
Cover in WRF-Chem on calculated aerosol (precursor) concentrations have not yet been reported.
In this study, we investigate the impact of the high resolution
Shuttle Radar Topography Mission (SRTM) 90 90 m topography
data (Farr et al., 2007; Jarvis et al., 2008) together with the
100 100 m resolution Corine Land Cover 2006 (Heymann et al.,
1994; Bttner et al., 1998, 2002) on the simulated gas and particulate matter (PM10) concentrations by WRF-Chem. In order to
investigate the impact of the SRTM and Corine Land Cover we
compare the simulated concentrations with the results of the WRFChem simulation using the standard 30-arc seconds United States
Geological Survey (USGS) Land Cover and topography (Anderson
2. Methodology
The WRF model is used over a part of the Italian/Swiss Alps and
the Po Valley area (northern Italy) to study the impact of high
resolution SRTM topography and Corine Land Cover on the simulated gas and PM10 concentrations. More details regarding WRFChem are given in Section 2.1. WRF-Chem operates on the
10 10 km and 2 2 km resolution. Fig. 1 presents the
geographical position of the model grid domains The
10 km 10 km domain (approximately 1100 km 950 km centred
at 8.603 longitude and 45.916 latitude) covers the Eastern part of
France, southern part of Germany, Switzerland, a large part of Italy
including a part of the Adriatic Sea and Mediterranean Sea. Domain
2 (approximately 300 km 200 km) covers a part of the Po Valley
in North Italy and the Southern part of Switzerland.
The two simulations were performed with no nudging to the
observations of the meteorological stations. The rst simulation
uses the SRTM and Corine Land Cover data for January 2010. The
second simulation uses the standard USGS 30-arc seconds land-use
data (~1 1 km) and topography data for the same period. The
simulation with SRTM and Corine Land Cover is further denoted as
WRF_CLC and the simulation with 30-arc seconds is further
denoted as WRF_USGS. For the simulations, a spin-up time of four
days is applied in order to initialize the model. WRF uses meteorological initial conditions and lateral boundary conditions from 6 h
analyses from the National Center for Environmental Protection
(NCEP; Kalnay et al., 1996), and the Climate Forecast System
Reanalysis (CFSR; Saha et al., 2010).
We start our study by evaluating the meteorological parameters
(temperature, wind speed and precipitation) calculated by
WRF_CLC and WRF_USGS. For more details we refer to De Meij and
Vinuesa (2014). Then we evaluate the calculated gas concentrations
of CO, SO2 and NOx and PM10 concentrations of both simulations.
Furthermore, we analyse the monthly mean calculated values of
the meteorological parameters and chemical species, together with
a more detailed evaluation of some selected episodes. For the
evaluation of the meteorological parameters and gas and PM10
concentrations we use observations of the Agenzia Regionale per la
Protezione dell' Ambiente (ARPA) network (www.arpalombardia.
it). An overview of the stations used and their geographical location is given in Table 1a. Through this website the following parameters can be downloaded: precipitation, temperature,
atmospheric pressure, wind speed and wind direction, relative
humidity, global irradiation and net irradiation. The statistical
analysis of the simulated meteorological values and gas concentrations in this work is based on hourly values. For PM10 that
analysis is based on daily mean concentrations. Depending on the
amount of observations available, the number of observedmodelled pairs differ from one station to the other.
The SRTM ew aboard the Space Shuttle Endeavour, which obtained terrain elevation data during an eleven day mission in
February of 2000 to generate the high-resolution (~90 m) digital
179
Fig. 1. Google Earth view of the two domains (D1 10 km 10 km, D2 2 km 2 km).
180
Table 1a
Overview of the stations used in this work and their geographical location in
longitude and latitude.
Table 1b
Overview of the WRF-Chem parameterisations, which are used for the 2 km 2 km
domain.
Station name
Longitude (degree)
Latitude (degree)
Parameter
WRF-Chem
Pavia
Gallarate
Osio Sotto
Treviglio
Bergamo via Meucci
Bergamo via Garibaldi
Calusco
Arese
Cassano d'Adda
Cinisello Balsamo
Legnano
Corsico
Limito
Milan viale Marche
Pero
Rho
Turbigo
Busto Arsizo, via Magenta
Somma Lombardo MXP
Varese via Vidoletti
Lallio
Costa Volpino
Cantu
Como
Erba
Mariano Comense
Olgiate Comasco
Colico
Lecco
Valmadrera
Moggio
Ospitaletti Brescia
Cormano
Saronno via Santuario
Casirate
Montanaso
Broletto
Darfo
Magenta
Sarezzo
Lodi via Vignati
Varese Voghera
9.15
8.79
9.58
9.59
9.88
9.66
9.47
9.07
9.51
9.21
8.91
9.11
9.33
9.19
9.08
9.04
8.73
8.85
8.70
8.80
9.63
10.10
9.13
9.08
9.22
9.18
8.96
9.36
9.39
9.36
9.48
10.07
9.16
9.02
9.56
9.46
10.21
10.18
8.88
10.20
9.50
9.01
45.05
45.66
45.62
45.52
45.61
45.69
45.69
45.55
45.52
45.55
45.59
45.53
45.50
45.49
45.51
45.53
45.53
45.61
45.68
45.84
45.66
45.83
45.73
45.80
45.81
45.70
45.78
46.13
45.85
45.85
45.93
45.55
45.54
45.62
45.49
45.33
45.54
45.88
45.46
45.65
45.31
44.99
6
10
18.5 km. The most relevant settings of WRF-Chem for domain 2 are
given in Table 1b.
WRF operates on two resolutions (10 10 km [D1] and 2 2 km
[D2]) following the NDOWN methodology (one way nesting). This
methodology involves using the coarse grid model simulation as
input for the ner model. The initial and lateral boundary conditions for the ner grid simulation are used from the coarse grid
simulation (ARW Users's Guide, http://www.mmm.ucar.edu/wrf/
users/docs/user_guide/ARWUsersGuide.pdf). In this work D2 uses
the lateral and boundary conditions from D1.
To investigate the impact of Corine Land Cover on calculated gas
and PM10 concentrations in WRF-Chem we run the D2 simulation
twice; once with the Corine Land Cover and once with the 30 arc
seconds USGS Land Cover.
The anthropogenic emissions are constructed for each domain
with the anthro_emis tool (available at http://www.acd.ucar.edu/
wrf-chem/download.shtml). The emissions used in the study are
from the EC-JCR/PBL (2010) Emissions Database for Global Atmospheric Research (EDGAR) inventory version 4.2 for the year 2008,
source: European Commission, Joint Research Centre (JRC)/
Netherlands Environmental Assessment Agency (PBL). Emission
Database for Global Atmospheric Research (EDGAR), release
version 4.2, http://edgar.jrc.ec.europa.eu, 2011. EDGAR v4.2 contains the following species CO2, CH4, N2O, HFCs, PFCs, SF6, CFCs,
Microphysics
Cumulus scheme
PBL
LSM
Surface Layer
Chemistry option
Chemistry time step
Photolysis scheme
Gas dry deposition
Aerosol dry deposition
Gas chemistry
Aerosol chemistry
Wet scavenging
Vertical mixing
Subgrid convective transport
Biomass burning emissions
Aerosol radiation feedback
(direct and indirect)
Yes (Noah)
Yes (Goddard)
Chou and Suarez (1999,
NASA Tech Memo)
WRF Single-Moment 5-class
scheme (Hong and Lim, 2006)
None
YSU (MRF successor) (Hong et al., 2006)
Noah (Chen and Dudhia, 2001)
Monin-Obukhov
GOCART coupled with RACM-KPP
1.5
Madronich photolysis (TUV)
Yes
Yes
Yes
Yes
None
Yes
Yes
None
None
HCFCs, CO, NOx, NMVOC, SO2, NH3, BC, OC, PM10 and PM2.5 on
0.10 0.10 (Olivier et al., 2001; Janssens-Maenhout et al., 2012).
The emissions depend on type of activities, seasonal and
geographical distribution of the emissions and are based on information including urban/rural population density, animal density,
power and industrial plants, oil and gas elds, shipping and aircraft
routes, coal mines, road network, rice elds, crop and grass lands.
Sources of abrasive emissions in road transport and construction
are not included in the emission inventory, which are two important diffusive emission sources for PM10. Also absent are particulate matter emissions by wood burning for residential heating
purposes in northern Italy, and also biogenic emissions and secondary organic aerosol (SOA) formation. This is deemed acceptable
because the objective of this paper is to investigate the impact of
the high resolution SRTM topography and Corine Land Cover on
calculated air pollutants, and not to evaluate the model performance in air pollutant concentrations by comparison with
observations.
For our study we use PM10, PM2.5, SO2, NOx (as NO), NH3, CO,
CO2, OC, BC and CH4 total emissions. The emissions are distributed
in the lowest model layer, which is around 27 m. In De Meij et al.
(2009) two different emission inventories were used (EMEP and
AEROCOM) to study the impact of the vertical and temporal distribution of the emissions, it was found that most of the anthropogenic emissions are distributed in the rst model layer.
2.2. Differences in land-use between Corine Land Cover and USGS
Land Cover
To illustrate the differences in the land cover categories between
the Corine Land Cover and the 30s USGS data bases we show in
Fig. 2 the distribution of the 24 land cover classes.
A big fraction of the Po Valley in USGS is classied as Dryland
cropland and pasture, while in the Corine dataset several land
cover classes are represented, such as urban and built-up, deciduous broadleaf forest and cropland/woodland. Another difference is
found in the irrigated cropland and pasture, which in the Corine
181
Fig. 2. Geographical representation of the main land-use category classes in Corine Land Cover (a) and USGS (b) in the model domain.
182
Table 2
USGS 24 land use categories together with the number of cells per land use, in model
domain 2, for USGS and Corine Land cover.
USGS Land
use category
# Cells in the
USGS land use
# Cells in the
corine Land
cover
1
2
3
4
66
5541
141
e
277
2412
596
e
40
256
241
95
10
2
608
1
e
1116
566
267
e
e
e
e
932
3
e
393
e
615
508
e
42
e
953
e
e
602
186
122
e
e
1317
e
e
e
e
235
5
6
7
8
9
10
11
12
13
14
15
16
17
18
19
20
21
22
23
24
meteorological variables (wind speed at ten metres height, temperature at 2 m height [T2] and precipitation) in WRF was investigated. They compared the results with the WRF simulation using
the standard 30-arc seconds USGS Land Cover and topography, and
with observations of the ARPA network, with the focus on the
Lombardy region (north Italy) for a winter and a summer period in
2010. They used the same model conguration in WRF as this study,
with the only difference being that the domain of interest in this
study is larger and the horizontal resolution is 2 2 km, while in De
Meij and Vinuesa (2014) the domain had a horizontal resolution of
1 1 km.
3.1.1. Temperature at 2 m (T2)
De Meij and Vinuesa (2014) showed that during the winter
period large differences are found in calculated T2 between the two
simulations outside the city of Milan. WRF_USGS underestimated
the observed temperatures for seven (out of 20 stations), while
WRF_CLC underestimated the observations for 4 stations. In all
cases the relation RMSEmod < STDEVobs is valid, which is one of the
conditions for good quality modelling results (Barna and Lamb,
2000). In our study we nd similar differences in temperature
outside the city of Milan i.e. higher temperatures by WRF_CLC
(Fig. 3) due to the higher fraction urban built up area in the Corine
Land Cover, which is less present in the 30-arc seconds USGS
(Fig. 2). De Meij and Vinuesa (2014) found a large difference in the
fraction of urban built up for this area (~17 times higher in
CorineLC).
Over the Alps T2 by WRF_CLC are in general higher (up to ~3 C),
but there are also some areas for which WRF_CLC calculates lower
T2 than WRF_USGS (up to 3.5 C). Analysing the differences in the
terrain height between WRF_CLC (with SRTM) and WRF_USGS we
see that the differences in T2 follow the pattern of the differences in
the terrain height (Fig. 3c). Over the Alps, WRF_CLC calculates
higher temperatures (indicated in green, yellow and red) in areas
where the SRTM height is lower than USGS topography. Similar but
opposite, the areas within the black contour lines represent areas of
183
Fig. 3. Average temperatures at 2 m height (degrees Celsius) simulated by WRF_CLC (a) and WRF_USGS (b) for January 2010. Temperatures lower than 10 are indicated in blue
(minimum temperature is around 22 C for the two simulations) and temperatures higher than 6.5 are indicated in red. For WRF_USGS the maximum temperature is 6.9 C. In
Fig. 3c is the difference in monthly mean 2 m temperature (degrees Celsius) between WRF_CLC and WRF_USGS shown, together with the difference in height between SRTM and
USGS topography datasets (black contour lines). (For interpretation of the references to colour in this gure legend, the reader is referred to the web version of this article.)
184
Fig. 4. Monthly average sensible heat uxes by WRF_CLC (a) and WRF_USGS (b) in W/m2. The red colour represents SH uxes higher than 200 W/m2 and purple lower than 34 W/
m2. (For interpretation of the references to colour in this gure legend, the reader is referred to the web version of this article.)
We have seen that over the Po Valley region higher SH uxes are
in general calculated by WRF_CLC, due to the higher fraction of the
urban built-up class in the Corine Land Cover. Larger SH uxes
result in larger PBL heights (Van den Hurk, 1995) over the urban
areas, which corroborates the monthly average PBL heights by
WRF_CLC and WRF_USGS in Fig. 6. PBL heights are in general higher
for WRF_CLC than for WRF_USGS. This corresponds with the results
by De Meij and Vinuesa (2014). Higher PBL heights are calculated
over the Po and Ticino rivers by WRF_USGS, because higher sensible heat uxes are calculated for these areas as described earlier.
model domain than the 30-arc seconds USGS data the wind speeds
are reduced due to more friction. This conrms the nding by De
Meij and Vinuesa (2014). They found that the calculated average
wind speeds are in general lower by WRF_CLC than by WRF_USGS.
WRF_CLC predictions are in better agreement with the observations. For example, the bias of the average wind speeds predicted by
WRF_CLC is lower (0.70 0.33 m/s) than that predicted by
WRF_USGS (0.78 0.46 m/s). Similarly the STDERR values, based
on 8 stations, are on average lower by WRF_CLC (1.30) than by
WRF_USGS (1.38). All RMSE values are lower than the standard
deviation of the observed wind speeds.
SRTM topography shows slightly higher mountain peaks (up to
4015 m) than USGS topography (maximum is ~4009 m). The differences in terrain heights between SRTM and USGS are shown in
Fig. 8. Clearly visible from this gure are the differences in terrain
height over the Alps. Higher resolution of the topography by SRTM
(90 90 m) resolves better the mountains peaks, slopes and valleys, which impact the wind speeds (and direction) over complex
185
Fig. 5. Monthly average sensible heat uxes by WRF_CLC (a) and WRF_USGS (b) in W/m2. The red represents LH uxes higher than 100 W/m2 and purple lower than 10 W/m2.
(For interpretation of the references to colour in this gure legend, the reader is referred to the web version of this article.)
3.1.3. Precipitation
Over urban areas (e.g. city of Turin, Gallarate, city of Milan, and
the Bergamo area (Orio Sotto)) higher monthly total precipitation
are calculated by WRF_CLC (Fig. 8). The differences in higher precipitation over urban areas by WRF_CLC are related to the differences in the heat uxes and the related cloud liquid water. Cloud
liquid water over the Po Valley is larger for WRF_CLC varying between ~5 and 60% and over the Alps up to 70e80 % higher for some
places leading to more precipitation by WRF_CLC.
Fig. 8 shows also the differences in precipitation over the
domain. Analysing the differences in precipitation over the Alps by
overlaying the differences in height between the SRTM and USGS
topography (black contour lines) we see a clear pattern between
the differences in precipitation and those of height.
186
and Corine Land Cover than simulation with USGS, while the false
alarms values are in general similar. The frequency bias for the
threshold values 0.5 mm and 1.0 mm are larger than 1 for both the
simulations, indicating that they both overestimate the number of
precipitation events for these thresholds. Interesting is that for the
threshold value of 2 mm, lower FBI values are found for WRF_CLC at
the mountain stations (e.g. Como Villa Geno, Como Villa Gallia and
Caslino d'Erba). This result indicates a better timing in the precipitation events at these areas and is attributed to the implementation of the SRTM topography.
The Hansen-Kuipers score, which summarizes the model's
ability to correctly time both the precipitation events and to avoid
the false alarms, is in general 1% higher for WRF with SRTM and
Corine Land Cover. For the stations surrounded by complex terrain,
the maximum difference in HKS is found for Como Villa Gallia (31%,
2 mm threshold level). This indicates that WRF_CLC performs
better than WRF_USGS for the heavier precipitation events for this
station. The majority of the stations used in this work are located in
the Po Valley for which the differences in monthly precipitation
quantities between WRF_CLC and WRF_USGS are ~5 mm. The
average HKS is higher by WRF_CLC at six stations (out of 18) and by
WRF_USGS at 2 stations (out of 18). The larger monthly mean
Fig. 7. Monthly average wind speed (m/s) calculated by WRF_CLC (a) and WRF_USGS (b) for January 2010. The white pixels in WRF_USGS represent wind speeds up to 7.7 m/s.
Fig. 8. The differences in total monthly precipitation quantities between WRF_CLC and WRF_USGS. The black contour lines represent the differences in height between the SRTM
topography and the 30 arc seconds USGS topography (at 50 m).
188
Fig. 9. Difference of monthly average CO (a), NO (b) and SO2 (c) concentrations (ppmv) between WRF_CLC and WRF_USGS.
Gallarate
Pavia
Milan Verziere
Arese
Treviglio
Calusco d'Adda
Bergamo via Garibaldi
Cassono d'Adda
Corsico
Limito
Milan, viale Marche
Rho
Busto Arsizo, via
Magenta
Somma Lombardo MXP
Saronno, via Marconi
Como
Pavia via Folperti
Voghera
Average
0.59
0.65
1.78
1.31
1.65
0.85
1.93
1.49
1.66
1.06
1.99
1.60
1.12
0.47
0.25
0.50
0.48
0.42
0.33
0.51
0.29
0.47
0.36
0.46
0.50
0.49
0.24
0.15
0.43
0.37
0.22
0.22
0.22
0.24
0.39
0.34
0.45
0.34
0.25
0.10
0.05
0.20
0.17
0.11
0.08
0.08
0.12
0.19
0.18
0.21
0.15
0.10
0.24
0.14
0.42
0.36
0.22
0.22
0.21
0.24
0.39
0.33
0.44
0.35
0.25
0.09
0.05
0.20
0.15
0.10
0.09
0.08
0.12
0.18
0.17
0.21
0.15
0.10
0.55
0.63
2.20
1.00
0.66
1.26
0.37
0.44
0.72
0.22
0.24
0.42
0.21
0.31
0.22
0.12
0.13
0.27
0.09
0.14
0.09
0.03
0.04
0.12
0.21
0.31
0.21
0.11
0.12
0.27
0.09
0.12
0.08
0.11
0.03
0.12
Table 4
Monthly mean observed and calculated SO2 concentrations (ppb) by WRF_CLC and
WRF_USGS.
Station name
Gallarate
Lallio
Bergamo via Garibaldi
Treviglio
Colico
Como
Erba, via Battisti
Varese Vidoletti
Arese
Cassano d'Adda
Cinisello Balsamo
Corsico
Legnano
Cormano
Turbigo
Average
1.16
3.53
4.38
3.19
3.04
1.15
1.16
2.41
70.2
50.7
92.7
52.6
61.4
1.80
2.68
23.5
1.31
0.45
0.94
0.27
0.72
0.59
0.44
0.71
54.2
30.9
57.5
32.2
44.4
1.89
1.87
15.2
3.87
3.91
4.13
3.23
2.36
5.87
5.25
4.38
9.47
3.65
12.8
5.64
7.59
12.5
33.8
7.90
3.90
3.06
3.06
3.20
1.41
4.07
3.42
3.11
5.80
3.46
7.54
4.29
5.39
7.29
22.9
5.46
2.99
3.68
3.91
2.92
2.14
5.16
4.87
3.84
8.78
3.30
11.6
5.04
6.76
11.4
22.6
6.60
3.01
2.65
2.83
2.82
1.25
3.13
2.86
2.56
4.67
3.17
6.07
3.62
4.54
5.80
13.4
4.16
189
quantities of CO, SO2 and NO are found over urban areas such as
Turin, Milan, Pavia, Novara and north-west of Milan (not shown).
For CO, maximum differences in calculated monthly concentrations (WRF_CLC > WRF_USGS) are found around Turin, Milan
and Pavia (up to 0.038 ppmv, ~20% higher) and negative differences
(WRF_CLC < WRF_USGS) are found up to 0.026 ppm (~10% lower)
north of Turin. Comparing with observations, calculated monthly
mean CO concentrations are in general underestimated by a factor
of ~3.6 by both the simulations, respectively (based on 18 stations,
see Table 3). For both simulations, the temporal correlation coefcients are in general low, on average ~0.19.
A possible explanation for this large underestimation could be
related to frequent wood burning for heating purposes in Northern
Italy during the winter time, which are not accounted for in the
emission inventory. Uncertainties in the emission factors for CO in
the emission inventory and unaccounted sources of CO which
contribute to the underestimation of CO in the inventory could be
held responsible for the underestimation of CO in a winter period.
We emphasize that the objective of this study is to investigate the
impact of the high resolution SRTM topography and Corine Land
Cover on calculated air pollutants and not to evaluate the modelled
performance in calculated air pollutant concentrations by
comparing with observations.
For SO2 maximum differences are found also between Gallarate
and Novara up to 0.020 ppmv (~55%) and negative difference up
to 1.104 ppmv (~15%) between Pavia and Piacenza. Comparing
with observations (Table 4), calculated monthly mean SO2 concentrations are in general underestimated by a factor of ~2.9 and 3.6
by WRF_CLC and WRF_USGS, respectively For the stations which
are characterized as urban (e.g. Arese, Cassano d'Adda, Cinisello
Balsamo, Corsico and Legnano), the monthly mean observed values
are a factor of 9 and 10 higher than the calculated ones by WRF_CLC
and WRF_USGS, respectively. Interesting to note is that for these
locations, the monthly average SO2 calculated concentrations for
WRF_CLC is ~10% higher than for WRF_USGS. The large overestimation by the two simulations at Turbigo might be related to
the presence of the power plant in this area and the horizontal
distribution of the emissions in the emission inventory. The
representativity of the measurement location relative to the grid
cell of the model is always an issue when model results are
compared with ground-based measurements (De Meij et al., 2006).
The highest temporal correlation coefcients are found for Varese
Vidoletti; 0.45 for WRF_CLC and 0.33 for WRF_USGS. For the other
stations, the temporal correlation coefcients are low, on average
0.12. Excluding the urban stations and Turbigo from the comparison results in an underestimation by a factor of 1.5 and 1.8 for
WRF_CLC and WRF_USGS, respectively.
For NO, maximum differences are found between Gallarate and
Novara up to 0.017 ppmv (~50%) with negative differences (~20%)
found north of Turin. Compared to observations, calculated
monthly mean NOx concentrations are in general underestimated
by a factor of ~3.5 by the two simulations (based on 31 stations,
Table 5). On average, WRF_CLC calculates higher monthly mean
NOx values (~5%) than WRF_USGS for 12 (out of 29) stations, while
WRF_USGS calculates higher monthly mean NOx concentrations for
two stations. In general the temporal correlation coefcients by the
two simulations are low (~0.28) with the highest temporal correlation coefcient found for Colico by WRF_CLC (0.53).
As described earlier, the monthly mean CO concentrations by
the two simulations are very similar. However, analysing the
calculated CO concentrations for specic time periods we see larger
differences between WRF_CLC and WRF_USGS.
For example, in Fig. 10a the measured CO concentrations (ppm)
for Arese are shown, together with the calculated concentrations by
WRF_CLC and WRF_USGS. Arese is classied as urban built-up in
190
Table 5
Monthly mean observed and calculated NOx concentrations (ppm) by WRF_CLC and
WRF_USGS.
Station name
Pavia
Gallarate
Osio Sotto
Treviglio
Bergamo via Meucci
Bergamo via Garibaldi
Calusco
Arese
Cassano d'Adda
Cinisello Balsamo
Legnano
Corsico
Limito
Milan viale Marche
Pero
Rho
Turbigo
Busto Arsizo, via Magenta
Somma Lombardo MXP
Varese via Vidoletti
Lallio
Costa Volpino
Cantu
Como
Erba
Mariano Comense
Olgiate Comasco
Colico
Lecco
Valmadrera
Moggio
Average
0.06
0.09
0.07
0.06
0.08
0.10
0.11
0.10
0.07
0.13
0.09
0.07
0.08
0.12
0.13
0.10
0.06
0.06
0.06
0.06
0.09
0.06
0.10
0.11
0.06
0.11
0.08
0.03
0.09
0.05
0.01
0.08
0.02
0.07
0.04
0.03
0.06
0.07
0.07
0.08
0.04
0.08
0.06
0.05
0.05
0.07
0.09
0.07
0.04
0.05
0.05
0.04
0.07
0.03
0.06
0.07
0.05
0.08
0.06
0.02
0.06
0.04
0.01
0.01
0.01
0.02
0.02
0.02
0.01
0.02
0.02
0.04
0.02
0.05
0.03
0.03
0.03
0.04
0.04
0.03
0.04
0.03
0.02
0.02
0.02
0.01
0.02
0.02
0.02
0.03
0.02
0.01
0.02
0.01
0.01
0.02
0.01
0.01
0.01
0.01
0.00
0.01
0.01
0.02
0.02
0.03
0.01
0.02
0.02
0.02
0.02
0.02
0.02
0.01
0.01
0.01
0.01
0.00
0.01
0.01
0.01
0.01
0.01
0.01
0.01
0.01
0.01
0.01
0.01
0.02
0.02
0.02
0.01
0.02
0.02
0.03
0.02
0.05
0.03
0.03
0.03
0.04
0.04
0.03
0.03
0.03
0.02
0.02
0.02
0.01
0.02
0.02
0.02
0.03
0.02
0.01
0.02
0.02
0.01
0.02
0.01
0.01
0.01
0.01
0.01
0.01
0.01
0.02
0.01
0.02
0.01
0.02
0.02
0.02
0.02
0.02
0.02
0.01
0.01
0.01
0.01
0.00
0.01
0.01
0.01
0.01
0.01
0.01
0.01
0.01
0.00
0.01
3.3. PM10
Fig. 11 shows the difference in monthly average PM10 concentrations between WRF_CLC and WRF_USGS. The white lines
represent the height of the topographic from the SRTM dataset.
For the Po Valley area WRF_CLC calculates in general higher
monthly average PM10 concentrations, varying between ~1 mg/m3
(~3% higher) northerly of Milan to 2 mg/m3 (~7% higher) southerly of
Milan and 6.7 mg/m3 (~26% higher) westerly of Milan. Over a large
part of the Alps (indicated with the white terrain height contour
lines) WRF_USGS calculates higher monthly average PM10 concentrations (indicated in blue (in web version)) than WRF_CLC, but
the differences are small on average ~0.25 mg/m3 (up to ~20% lower
by WRF_CLC). An important removal mechanism for particulate
matter of the atmosphere is wet deposition. As mentioned in Section 3.1 large areas over the Alps show larger precipitation by
WRF_CLC, which removes the aerosol and precursors more effectively leading to lower monthly average PM10 concentrations than
by WRF_USGS. Similar to the distribution of the emissions of the
gas species, the highest PM10 emissions are found over Turin,
Milan, Pavia, Novara and the area north-west of Milan, which corroborates the presence of urban built-up area in the Corine Land
Cover, as mentioned previously.
Analysing the calculated PM10 concentrations in more detail,
we nd large differences between WRF_CLC and WRF_USGS,
especially during the night. In Fig. 12, we show for Busto Arsizio the
calculated PM10 concentrations by WRF_CLC and WRF_USGS
(dashed black and red lines, respectively) together with the PBL
heights for the two simulations (solid black and red lines, respectively). The city of Busto Arsizio (located ~<5 km south-easterly of
Gallarate) is classied as urban built-up in WRF_CLC and as dry
cropland and pasture in WRF_USGS.
The reason for the differences in PM10 concentrations is related
to the differences in PBL heights, especially during the night. For the
periods that WRF_CLC calculates higher PM10 concentrations the
PBL heights are lower than by WRF_USGS. For example, on 23rd
January higher PM10 concentrations are calculated by WRF_CLC
than by WRF_USGS (up to ~13 mg/m3 difference around 07:00GMT).
This difference is related to the lower PBL heights by WRFC_CLC.
The average PBL height during the night of 23 January (i.e. between
18:00 22nd January and 06:00 23rd January) by WRF_CLC is ~45 m
and ~143 m by WRF_USGS with a maximum difference of ~270 m
around 01:00 (GMT) on 23 January, see solid black and red lines in
Fig. 12. The differences in PBL heights are caused by the different
land cover classications and the related heat uxes. As described
before, sensible heat uxes are responsible for the development of
the PBL heights. Corresponding average sensible heat uxes
are 0.02 W/m2 for WRF_CLC and 7.3 W/m2 for WRF_USGS during
this period, which are related to the differences in land cover
classications as mentioned before.
The difference in PBL heights is responsible for the differences in
aerosol concentrations between WRF_CLC and WRF_USGS. During
the night of 23 January the vertical mixing by WRF_USGS is better
than by WRF_CLC, because of the higher PBL height. A deeper PBL
leads to lower aerosol concentrations at ground level. Daily average
PM10 observed concentration for Busto Arsizio on 23rd January is
66 mg/m3 and calculated averages are 32.6 mg/m3 by WRF_CLC and
23.5 mg/m3 by WRF_USGS.
A quantitative comparison of the monthly average PM10 concentrations with the observations shows that calculated PM10
concentrations are underestimated by a factor ~4 by the two simulations (see Table 6). As mentioned in Section 2 the absence of
abrasive road and construction diffusive PM10 emissions in the
EDGAR emission inventory, the absence of PM emissions by wood
burning for residential heating purposes in northern Italy, the
absence of biogenic emissions and the absence of SOA formation
contribute to the underestimation of the calculated PM10 concentrations. Nevertheless, on this day WRF_CLC calculates higher PM10
concentrations than by WRF_USGS due to the impact of the
improved resolution brought by the Corine Land Cover and is closer
to the observations. A study by De Meij et al. (2009) found also a
large underestimation of calculated PM10 concentrations over the
Po Valley during a winter period. Monthly mean calculated PM10
concentrations were underestimated by a factor of ~3 for January
2005 when compared to observations (based on 5 stations).
On average WRF_CLC calculates higher monthly mean average
PM10 concentrations (3.5%) than WRF_USGS for 15 (out of 25)
stations. The largest differences are calculated for Turbigo (13.8%),
Voghera (14.2%) and Montanaso (8%). For 12 (out of 25) stations, the
191
(a)
(b)
Fig. 10. (a) Measured hourly CO concentrations (ppm) for Arese (black line) together
with the calculated concentrations by WRF_CLC (red line) and WRF_USGS (blue line)
for January 2010. (b) Snapshot of the calculated CO concentrations together with the
calculated wind speeds for the period 22 and 23 January. The solid lines represent the
calculated CO concentrations by WRF_CLC (black) and WRF_USGS (red), the dashed
lines the corresponding wind speeds by the two simulations. The right y-axis in (b)
represents the wind speed in m/s. (For interpretation of the references to colour in this
gure legend, the reader is referred to the web version of this article.)
Fig. 12. PM10 concentrations by WRF_CLC and WRF_USGS for Busto Arsizio (black and
red dashed lines, respectively), together with the PBL heights for the two simulations
(WRF_CLC black; WRF_USGS red) for 2 days in January (22nde24th January). Right yaxis represents the PBL height in meters. (For interpretation of the references to colour
in this gure legend, the reader is referred to the web version of this article.)
Fig. 11. The difference in monthly average PM10 concentrations (mg/m3) between WRF_CLC and WRF_USGS. The white lines represent the terrain height of the topographic by the
SRTM dataset.
192
Table 6
Monthly mean observed and calculated PM10 concentrations (mg/m3) for WRF_CLC
and WRF_USGS.
Station name
Busto Arsizio
Gallarate Piazza
S. Lorenzo
Saronno via Santuario
Calcuso d'Adda
Casirad d'Adda
Osio Sotto
Treveglio
Cantu via Meucci
Erba via Battisti
Olgiate Comasco
Arese
Magenta
Milano Verziere
Lodi viale Vignati
Montanaso
Bergamo via Garibaldi
Lallio
Moggio
Valmadrera
Lecco
Varese Copelli
Voghera
Turbigo
Limito
Cassano d'Adda
Average
63.3 27.9
67.9 33.3
76.2
65.1
73.2
59.3
66.0
50.9
55.6
59.9
71.3
59.4
74.8
64.3
58.6
78.3
71.4
11.3
63.9
54.2
56.8
58.2
60.2
77.2
84.1
63.3
35.6
27.1
23.3
25.8
23.3
22.6
29.5
25.5
30.7
24.1
30.3
27.2
21.8
32.8
27.4
7.24
31.1
30.6
24.7
24.3
24.9
30.8
27.9
26.8
17.1 6.55
16.1 6.17
18.0
18.2
14.4
15.3
14.3
15.7
12.9
14.1
21.4
17.6
22.5
16.5
16.0
13.9
14.6
8.51
12.3
14.5
14.0
11.2
23.0
18.7
15.5
15.9
7.05
5.68
5.91
5.77
6.12
5.74
4.90
5.32
7.65
6.71
7.71
5.90
4.93
4.84
5.18
3.79
4.68
5.31
5.34
4.22
8.48
7.50
6.06
5.90
17.0 6.40
16.1 6.13
17.8
18.2
13.8
15.0
14.1
15.5
12.5
14.0
21.3
17.3
22.1
16.2
14.8
13.5
14.4
8.69
12.9
14.4
14.2
9.80
20.2
19.1
15.2
15.5
6.72
6.14
5.80
5.78
5.99
5.46
4.90
5.20
7.44
6.64
8.19
5.90
5.44
5.01
5.18
3.84
5.01
5.40
5.10
4.30
7.93
8.13
6.25
5.93
are around 39.5 and 44.9 W/m2, respectively and mean LH uxes
are 19.2 and 22.0 W/m2, respectively.
4. Conclusions
In this paper, we investigated the impact of using SRTM
topography data together with Corine Land Cover on the simulated
gas and PM10 by WRF-Chem. We focused our analysis on the wellknown, highly urbanized region of the Po Valley in northern Italy.
Our analysis was performed by comparing the results to a simulation using topographic and land cover USGS data, resolved to 30 arc
seconds and observations.
Our analysis conrms the previous ndings of De Meij and
Vinuesa (2014). Specically, large differences in the geographical
Fig. 13. PM10 concentrations by WRF_CLC and WRF_USGS for Osio Sotto (black and
red dashed lines, respectively), together with the PBL heights for the two simulations
(WRF_CLC black; WRF_USGS red) for 2.5 days in January (16the18th January). Right yaxis represents the PBL height in meters. (For interpretation of the references to colour
in this gure legend, the reader is referred to the web version of this article.)
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