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Several methods were used for the efficiency calibration of a counting system
ORTEC PROTEAN MPC-2000-DP by using KCl reference samples (reference sources
of naturally radioactive potassium chloride), along with 241Am and 90(Sr-Y) radioactive
sources. The operations were part of gross alpha and beta counts in various samples at
the IFIN-HH SALMROM Laboratory specializing in the spectroscopic survey of the
environment and radioactive materials.
Key words: gross alpha and beta counter, calibration, gross alpha/beta counts.
1. INTRODUCTION
We used a fixed geometry in metallic sample trays, in the MPC 2000 lead
shield, directly facing the detector probe; two counting geometries were used:
Rom. Journ. Phys., Vol. 56, Nos. 34, P. 373387, Bucharest, 2011
374
SAMPLE
SAMPLE CODE
1
2
3
4
5
6
7
8
9
10
11
12
13
14
15
sample 1 - CPR
sample 2 - CPR
sample 3 - CPR
sample 4 - CPR
sample 5 - CPR
sample 6 - CPR
sample 7 - CPR
sample 1 - DFVM
sample 2 - DFVM
sample 3 - DFVM
sample 4 - DFVM
sample 5 - DFVM
sample 6 - DFVM
sample 7 - DFVM
empty tray
WEIGHT
(g)
0.4004
0.5003
0.6002
0.7004
0.8003
0.9000
1.0000
0.4028
0.5028
0.6028
0.7028
0.8028
0.9028
1.0028
0.0000
ERROR
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0000
375
EXPERIMENTAL RESULTS
The samples were measured, and the characteristic calibration curve of the
detector was drawn (Graphs 1 and 2) with the help of the PICPLAT_KCl01
(PICPLAT_KCl_GRAPH) file from the calibration folder of the measuring
system. The graphs were made with the EXCEL software, according to table 2 (x
axis the power tension of the detector; y axis registered the events).
Thus we obtained:
Table 2
Counts = f (U)
DP Detector
Plateau Data
VOLTS (V)
705
720
735
750
765
780
795
810
825
840
855
870
885
900
915
930
945
960
975
990
1005
1020
1035
1050
1065
1080
PIC MPC2000BDP
COUNTS
1
8
22
58
138
317
541
947
1548
2222
3009
4053
5140
6341
7753
8996
10252
12432
14127
16620
19581
22276
25093
27722
28698
29495
SLOPE(%/100
volts)
0
0
0
0
0
97.54
83.09
71.57
62.53
55.23
49.22
44.43
40.49
36.7
33.37
31.39
29.47
28.33
27.33
25.88
24.62
22.96
20.56
17.65
13.3
8.32
376
4
Table 2 (continued)
1095
1110
1125
1140
1155
1170
1185
1200
1215
1230
1245
1260
1275
1290
29585
29914
29587
29578
29884
30138
30078
29808
30126
30463
30211
30077
30329
30439
4.16
0.37
0.57
1.55
2.98
1.37
0.34
1.44
1.85
1.29
0.04
0.15
0
0
COUNTS
35000
30000
25000
20000
15000
10000
5000
0
700
800
900
1000
1100
1200
1300
1050
1100
1150
1200
1250
1300
377
The point-like sources of 241Am and 90(Sr-Y) were also measured and then
the file of mesuring data was established: PICDATA_KCL01_FINAL ULTERIOR
PROCESSING OF MEASUREMENTS DONE FOR STANDARDIATION/
CALIBRATION (table 8) from the calibration folder of the measuring system.
This folder containing the data got by the specialized software PIC Comunicator
carries all the characteristic parameters of the system and it was the source of the
experimental data used in the standardization report and in the report regarding the
validation of the word procedure. The measuring data was studied in conformity
with the folder PICDATA_KCL01_FINAL (PICDATA_KCL01, KCL_BETA
Weight of the made ethalon sample-1, sample-2, sample-3: The influence of the
samples weight The autoabsorbtion correction and the influence of the operator
who is preparing the refence samples. The experimental data obtained in this way
are in conformity with the technical data and the specifications of the system and
the detection eficiency for the alfa, beta and Spillover factor Xtalk were calculated
with the formulas below and are present in Table 3 and 4.
=
=
CPM FondCPM
DPM
X talk =
CPM FondCPM
CPM FondCPM
100;
For the measuring of the samples and the radiation sources the two methods of
work were used:
Measuring geometry I
378
Table 3
Detection efficiencies in measure I geometrics
SURCE/Radionucleid
SI
(imp/s)/Bq=
(imp/min)/(dez/min)=
(CPM)/(DPM)
0,89872
0,0138
imp/( in 2)
0,44936 0,0069
0,62730
0,0050
imp/( in 2)
0,31365 0,0025
= 31,365
0,25
0,2559 0,0050
25,59 0,50
Detection
efficiences
(% )MPC2000
= 44,936
0,69
Measuring geometry II
SI
(imp/s)/Bq =
(imp/min)/(dez/min)=
(CPM)/ (DPM)
0,89872
0,0138
imp/( n 2)
0,4853 0,0074
0,80574
0,0142
imp/( in 2)
0.40287
40,2870,71
0,7246
0,0058
imp/( in 2)
0,3623 0,0029
= 36,23
0,29
0,3108 0,006
31,08 0,60
Detection
efficiences
(% )MPC2000
= 48,53
0,74
379
-18.064
50.044
The influence of the sample mass and the autoabsorbtion correction on the
measurements is also set out in the EXCEL standardization file:
PICDATA_KCL01_FINAL/probe 2. The general medium error (% relative),
maximum error (% relative), minimum error (% relative), maximum error for the
neglection of the autoabsorbtion correction for averages and maximum error for
the neglection of the autoabsorbtion correction for all points have also been
calculated (as shown in Table 6).
380
1.
2.
Detectable beta
activity, ALFA +
BETA SUS routine
90
(Sr-Y) SEB 7-4673
Source/
MPC 2000 System
Routine detectable
alfa activity ALFA
+ BETA SUS
241
Am SEA 4-1
Source/ MPC 2000
System
Results
Activity [Bq]
Measurement uncertainty
SALMROM
LAS
SALMROM
LAS
Uncertaint
y[Bq]
7.01x103
6.78 x103
251
1.38x104
1.43 x104
Err (%)=-11.53%
425
ELEME
NT
H
ATOMIC MASS
Table 7
0.672
4.190
-4.316
-1.104
1.339
-3.528
-2.403
-1.410
-1.710
0.323
3.119
0.217
1.029
3.113
REL. ERR
towards
FIT [%]
g KCl /
0.0001 SAMPLE==
ERROR
MASUREM
ENT
MASS
-4.316
-4.316
-4.316
-4.316
-4.316
-4.316
-4.316
MAX ERR
[%]
OPERATOR 2 = DFVM
10 g KCl / Sample==
50 g KCl / Sample==
100 g KCl / sample==
INTRODUCES VALUE
MASS===>
NR.de ATOMI
KCl
43.690
42.378
41.176
40.080
39.097
38.225
37.460
OPERATOR 1= CPR
43.074
41.654
41.309
41.330
39.182
38.618
38.626
OPERATOR 2 = DFVM
BEFF
CURVE
[%]
FIT gr.2
POTASSYUM CHLORIDE
AVERAGE======== >
43.983
44.154
39.399
39.638
39.621
36.876
36.560
FORMULA====>
SUBSTANCE
MASS
0.400
0.500
0.600
0.700
0.800
0.900
1.000
BEFF [%]
OPERATOR 1= CPR
Table 6
Yield BETA
40-K
89.33 %
4.190
4.190
4.190
4.190
4.190
4.190
4.190
MIN ERR.
[%]
Table 7 (continued)
0.5003
0.5003
0.6002
0.6002
0.6002
0.6002
0.6002
0.6002
0.7004
0.7004
0.7004
0.7004
0.7004
0.7004
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
434.8513
434.8513
521.6825
521.6825
521.6825
521.6825
521.6825
521.6825
608.7744
608.7744
608.7744
608.7744
608.7744
608.7744
0.737%
0.737%
0.734%
0.734%
0.734%
0.734%
0.734%
0.734%
0.731%
0.731%
0.731%
0.731%
0.731%
0.731%
45.434
45.756
38.255
38.907
39.175
40.057
40.095
39.904
40.306
39.156
37.185
40.568
39.977
40.634
1.649
1.654
1.382
1.389
1.393
1.408
1.407
1.405
1.294
1.277
1.249
1.298
1.288
1.298
12.77
13.57
-5.04
-3.43
-2.76
-0.57
-0.48
-0.95
0.05
-2.81
-7.70
0.70
-0.77
0.86
BEFF_ERR
MASS ERR_MASS ACTIVITY ERR_ACT BEFF
Gen Avg ERR
_absolut
[g]
[g]
[DPM]
[%]
[%]
[% relativ]
[%]
0.4004
0.0001
348.0201
0.742%
44.989
1.872
11.67
0.4004
0.0001
348.0201
0.742%
44.701
1.865
10.96
0.4004
0.0001
348.0201
0.742%
41.828
1.816
3.82
0.4004
0.0001
348.0201
0.742%
43.610
1.848
8.25
0.4004
0.0001
348.0201
0.742%
44.587
1.866
10.67
0.4004
0.0001
348.0201
0.742%
44.184
1.856
9.67
0.5003
0.0001
434.8513
0.737%
43.088
1.612
6.95
0.5003
0.0001
434.8513
0.737%
42.398
1.602
5.24
0.5003
0.0001
434.8513
0.737%
44.054
1.627
9.35
0.5003
0.0001
434.8513
0.737%
44.192
1.629
9.69
1.20
39.399
0.7447414
1.89
0.3040394
0.77
39.638
1.3168505
3.32
0.537602
1.36
S[AVERAGE]=[%]==>
AVERAGE ======= >
S[n-1]========>
S[n-1]===[%]===>
S[AVERAGE]=====>
S[AVERAGE]=[%]==>
AVERAGE ======= >
S[n-1]========>
S[n-1]===[%]===>
S[AVERAGE]=====>
S[AVERAGE]=[%]==>
44.154
AVERAGE ======== >
1.2987282
S[n-1]========>
2.94
S[n-1]===[%]===>
0.5302036
S[AVERAGE]=====>
43.983
AVERAGE ======== >
1.1589448
S[n-1]========>
2.63
S[n-1]===[%]===>
0.4731372
S[AVERAGE]=====>
1.08
S[AVERAGE]=[%]==>
1.07
1.15
1.18
1.29
[% relative]
S[POISSON]
Table 8
-1.61
-2.21
9.60
9.17
ERROR
ACTIVITY
AVERAGE ON
MED=40.287
S[n-1]=2.391073
S[n-1]=[%]=5.94
S[AVERAGE]=0.639041
S[AVERAGE][%]=1.586
S[n-1] = 2.612765
S[n-1] [%]=6.49
S[AVERAGE]=0.285076
S[AVERAGE] [%] =0.71
AVERAGE =40.28
0.8003
0.9000
0.9000
0.9000
0.9000
0.9000
0.9000
1.0000
1.0000
1.0000
1.0000
1.0000
1.0000
0.4028
0.4028
0.4028
0.4028
0.4028
0.4028
0.5028
0.5028
0.5028
0.5028
0.5028
0.5028
0.8003
0.8003
0.8003
0.8003
0.8003
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
695.6056
782.2630
782.2630
782.2630
782.2630
782.2630
782.2630
869.1811
869.1811
869.1811
869.1811
869.1811
869.1811
350.1061
350.1061
350.1061
350.1061
350.1061
350.1061
437.0242
437.0242
437.0242
437.0242
437.0242
437.0242
695.6056
695.6056
695.6056
695.6056
695.6056
0.729%
0.728%
0.728%
0.728%
0.728%
0.728%
0.728%
0.727%
0.727%
0.727%
0.727%
0.727%
0.727%
0.742%
0.742%
0.742%
0.742%
0.742%
0.742%
0.737%
0.737%
0.737%
0.737%
0.737%
0.737%
0.729%
0.729%
0.729%
0.729%
0.729%
39.731
36.608
35.790
37.784
36.071
37.656
37.349
37.963
38.447
36.076
35.708
35.225
35.938
39.122
44.035
42.778
44.949
40.094
47.463
41.135
41.089
42.188
41.089
42.691
41.730
39.932
40.565
40.220
37.661
39.616
1.195
1.080
1.069
1.096
1.072
1.095
1.090
1.039
1.045
1.014
1.008
1.002
1.012
1.764
1.849
1.828
1.863
1.783
1.906
1.577
1.576
1.593
1.576
1.601
1.586
1.198
1.206
1.203
1.166
1.193
-1.38
-9.13
-11.16
-6.21
-10.47
-6.53
-7.29
-5.77
-4.57
-10.45
-11.37
-12.57
-10.79
-2.89
9.30
6.18
11.57
-0.48
17.81
2.10
1.99
4.72
1.99
5.97
3.58
-0.88
0.69
-0.17
-6.52
-1.67
39.621
1.0198493
2.57
0.4163517
1.05
36.876
0.8434348
2.29
0.3443308
0.93
36.560
1.3157308
3.60
0.5371449
1.47
43.074
3.1076325
7.21
1.2686857
2.95
41.654
0.6742501
1.62
0.2752615
0.66
3.39
6.92
-9.25
-8.47
-1.65
Table 8 (continued)
1.01
0.99
0.95
1.29
1.20
0.6028
0.6028
0.6028
0.6028
0.6028
0.6028
0.7028
0.7028
0.7028
0.7028
0.7028
0.7028
0.8028
0.8028
0.8028
0.8028
0.8028
0.8028
0.9028
0.9028
0.9028
0.9028
0.9028
0.9028
1.0028
1.0028
1.0028
1.0028
1.0028
1.0028
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
523.9424
523.9424
523.9424
523.9424
523.9424
523.9424
610.8605
610.8605
610.8605
610.8605
610.8605
610.8605
697.7786
697.7786
697.7786
697.7786
697.7786
697.7786
784.6967
784.6967
784.6967
784.6967
784.6967
784.6967
871.6148
871.6148
871.6148
871.6148
871.6148
871.6148
0.733%
0.733%
0.733%
0.733%
0.733%
0.733%
0.731%
0.731%
0.731%
0.731%
0.731%
0.731%
0.729%
0.729%
0.729%
0.729%
0.729%
0.729%
0.728%
0.728%
0.728%
0.728%
0.728%
0.728%
0.727%
0.727%
0.727%
0.727%
0.727%
0.727%
40.266
41.640
40.953
43.091
39.693
42.213
41.085
40.397
40.070
42.362
42.427
41.641
39.578
38.260
40.754
38.317
39.034
39.149
36.673
39.018
40.394
38.610
38.431
38.584
39.464
38.775
38.018
37.788
38.890
38.821
1.408
1.428
1.418
1.450
1.397
1.436
1.302
1.293
1.288
1.320
1.322
1.311
1.190
1.173
1.206
1.173
1.183
1.184
1.079
1.110
1.129
1.106
1.103
1.104
1.056
1.047
1.038
1.036
1.049
1.048
-0.05
3.36
1.65
6.96
-1.47
4.78
1.98
0.27
-0.54
5.15
5.31
3.36
-1.76
-5.03
1.16
-4.89
-3.11
-2.83
-8.97
-3.15
0.26
-4.16
-4.61
-4.23
-2.04
-3.75
-5.63
-6.20
-3.47
-3.64
41.309
1.2590249
3.05
0.5139948
1.24
41.330
0.9882595
2.39
0.4034553
0.98
39.182
0.9217383
2.35
0.3762981
0.96
38.618
1.1944575
3.09
0.4876352
1.26
38.626
0.6168569
1.60
0.2518308
0.65
0.93
0.97
1.02
1.05
1.12
-4.12
-4.14
-2.74
2.59
2.54
Table 8 (continued)
0.001
0.001
0.001
0.001
0.001
0.001
0.0001
0.0001
0.0001
0.0001
0.0001
0.0001
0.8692
0.8692
0.8692
0.8692
0.8692
0.8692
1.072E-01
1.072E-01
1.072E-01
1.072E-01
1.072E-01
1.072E-01
210.543
387.721
348.604
663.843
111.599
-95.492
-347.111
384.065
-339.493
392.190
399.654
-320.892
AVERAGE======== >
S[n-1]========>
S[n-1]===[%]===>
S[AVERAGE]=====>
S[AVERAGE]=[%]==>
84.754
383.49508
452.48
156.56121
184.72
Table 8 (continued)
2.60
15
387
5. CONCLUSIONS
The results which were obtained in the SALMROM laboratory from the
measuring/ testing/rating and comparison data validate the use of the measuring
method, pointing out that the MPC 2000 system is correctly calibrated in
efficiency, while observing the processed testing geometries.
The system can be used for:
Measuring radioactive alfa and beta concentrations in a wide range of
different samples: solid, liquid, filtres, aerosoles etc.;
Monitoring radioactive alfa and beta concentrations in the environment,
biological and food samples, mineral and geological samples, radioactive
waste, materials used in the nuclear industry and its applications;
Characterization of the content of total alfa and beta radionucleids in
different samples and screening for the selection of special samples, etc.
REFERENCES
1. Halbwertszeiten und Photonen-Emissionswahrscheinlichkeiten von hufig verwendeten Radionukliden2005 eiwerterte und korrigierte Auflage von Ulrich Schtzig und Heinrich Schrader PhysikalischTechnische Bundesanstalt (PTB), Braunschweig.
2. SR EN ISO/CEI 17025: 2005 Cerine generale pentru competena laboratoarelor de ncercri i
etalonri.
3. Legea 111/1996 privind desfurarea n siguran a activitilor nucleare, republicat, cu
modificrile i completrile ulterioare.
4. Manualul Calitatii al IFIN-HH, MC-00-00, ediia n vigoare.
5. Manualul Calitatii al SALMROM, MC-FVM-100, Rev. 1, 2009, ediia n vigoare.
6. Manualele de operare, documentaia tehnic Sistem de masur a radioactivitii alfa i beta
globale n fond sczut model MPC 2000.
7. Precedures manual, Environmental Measurements Laboratory, HASL - 300, U S Department of
Energy, 1992.
8. Raport de Etalonare al sistemului MPC 2000, nr. 2/2008, Cod: RE-FVM-101B, Nr. 2/2009.
9. IAEA - Update of X Ray and Gamma Ray Decay Data Standards for Detector Calibration and
Other Applications, Volume 1: Recommended Decay Data, High Energy Gamma Ray Standards
and Angular Correlation Coefficients, 2007.
10. IAEA - Update of X Ray and Gamma Ray Decay Data Standards for Detector Calibration and
Other Applications, Volume 2: Data selection, Assessment and Evaluation Procedures, 2007.