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Ultrasonics Sonochemistry
journal homepage: www.elsevier.com/locate/ultsonch
a r t i c l e
i n f o
Article history:
Received 6 October 2009
Accepted 8 November 2009
Available online 18 November 2009
Keywords:
Power ultrasound
Transducers
Industrial processing
a b s t r a c t
High-power ultrasonics (HPU) is a green emerging technology that offers a great potential for a wide
range of industrial processes. Nevertheless such potential have remained restricted during many years
to a limited number of applications which reached commercial development. The possible major problem
for extending the range of HPU industrial applications has been the lack of power ultrasonic transducers
for large-scale application, adapted to the requirements of each specic problem with high efciency and
power capacity.
A new family of HPU transducers with extensive radiators have been recently introduced. It comprises
a variety of transducer types designed with the radiators adapted to different specic uses in uids and
multi-phase media. Such transducers implement high power capacity, high efciency and radiation pattern control. In addition, their design incorporate strategies to eliminate or reduce modal interactions
produced at high power as a consequence of their nonlinear behaviour. The introduction of such new
transducers has signicantly contributed to the development at semi-industrial and industrial level of
a number of processes in the food and beverage industry, in environment and in manufacturing. This
paper deals with the basic structure and main characteristics of such transducers as well as their performance in the developed application processes.
2009 Elsevier B.V. All rights reserved.
1. Introduction
The development of green technologies for industrial processing is at present one of the main scientic and technological
challenges. High-power ultrasonics (HPU) is a green emerging
technology that offers a great potential for a wide range of processes. HPU technology is based on the application of high-intensity elastic waves to cause changes in the treated media by the
adequate exploitation of the nonlinear phenomena associated to
the high amplitudes such as radiation pressure, wave distortion,
streaming, and cavitation in liquids and dislocation in solids. As a
consequence, a series of mechanisms can be activated by the ultrasonic energy such as agitation, diffusion, interface instabilities, friction reduction, localised heating, mechanical rupture, chemical
effects etc. Such mechanisms can be exploited to produce or to enhance industrial processes.
Important features of HPU technology, besides its green and
sustainable character, are its capacity to act synergistically with
other forms of energy in order to promote, accelerate or improve
existing processes as well as its ability to produce different effects
in different media.
The idea of using ultrasonic energy in industry has been explored since the rst half of the 20th century. HPU systems for
* Corresponding author.
E-mail address: jgallego@ia.cetef.csic.es (J.A. Gallego-Jurez).
1350-4177/$ - see front matter 2009 Elsevier B.V. All rights reserved.
doi:10.1016/j.ultsonch.2009.11.006
954
such as food industry, environment, pharmaceuticals and chemicals manufacture, machinery, etc. In the last fteen years, the advent of powerful nite element modelling packages, the
development of electronic methods to drive and control tuned
oscillating systems [1] and the need of green technologies for
industrial processing, have all contributed to revive the interest
in HPU.
The recent introduction of a new family of HPU transducers
with extensive radiators, which comprises a variety of types designed for specic uses in uids (especially gases) and multi-phase
media, has strongly contributed to the implementation at semiindustrial and industrial stage of several commercial applications,
in sectors such as food industry, environment and manufacturing.
This article deals with the structure and characteristics of the main
transducer types of this family as well as their performance as an
innovative technology in several industrial processes.
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do zo
1
di zo hi r2i 2
di di1
k
2
Fig. 3. Comparison between the directivity patterns of a at-plate radiator and a directional stepped-plate radiator.
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Table 1
Main characteristics of directional circular stepped-plate transducers.
Electroacoustic efciency
Directivity (3 dB beam width)
Power capacity
Frequency range experimented
Maximum intensity levels
7580%
<2
1 kW
1040 kHz
175 dB
these transducers is very similar to that of the directional transducers of the same diameter. Fig. 7 shows the acoustic eld of a
focusing circular plate transducer with a plate radiator of 39 cm
in diameter and an operating frequency of 25.8 kHz. The ultrasonic
energy is concentrated in a focal volume of about 2 cm in diameter
and 17 cm in length (dimensions taken at 3 dB of the maximum value) located at a distance of about 40 cm from the plate radiator.
Intensities of the order of 170 dB are obtained in the focus with a
power applied to the transducer of 200 W.
3.1.4. The rectangular stepped-plate transducer
For specic industrial applications, the stepped-plate transducers with rectangular radiating surface offer technical and practical
advantages over transducers with circular radiators. Rectangular
plate congurations allow a more uniform distribution of vibration
displacements than circular plates. In fact the distribution of displacements of axisymmetric circular plate vibrators, given by Bessel functions, presents high amplitudes in the inner area and much
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ural mode of the plate radiator, together with the high modal density of rectangular vibrating plates, make these transducers more
sensitive to exhibit nonlinear response characteristics when driven
at high power.
The rectangular radiators have been designed to operate in a
resonant mode with 14 nodal lines parallel to its smaller side. Both
faces of the radiator are stepped to obtain directional radiation also
from the back face. The purpose is to use the back radiation in the
forward direction by means of adequate reectors. Prototypes for 7
and 20 kHz have been developed with power capacities up to
2.7 kW (Fig. 9). The main characteristics measured in air are shown
in Table 2. The directivity patterns are shown in Fig. 10.
3.2. The grooved-plate transducer
The performance of the industrial transducers very much depends on their behaviour under high strain levels. Amongst the
power limitations of the industrial use of HPU devices, two are
the more important issues to be considered: one is related with
Fig. 8. Comparison of amplitude distribution between circular and rectangular vibrating plates.
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Table 2
Main characteristics of the directional rectangular stepped-plate transducers.
Radiating
plate (m2)
Frequency
(kHz)
Bandwidth
(Hz)
1.8 0.8
0.6 0.3
7.6
19.5
1
2.5
Directivity
(3 dB beamwidth)
XZ plane
about 2
about 2
Efciency
(%)
YZ plane
67
75
the difculties to reach very high powers without nonlinear disturbances and the other refers to the distribution and location of the
stresses to maximize the power capacity of the transducers.
HPU transducers reveal a common feature due to their inherent
nonlinear vibration characteristics which frequently hamper the
industrial use of the ultrasonic technology. As well known, tuned
transducers when driven at high power levels exhibit a range of
nonlinear phenomena and their response generally includes harmonics of the driving frequency and, when the amplitude exceeds
a threshold level and under certain conditions, such response may
also contain fractional harmonics, frequency pairs, combination
resonances, frequency modulations, etc. As a result, high-power
operation of complex transducers, designed to resonate in a tuned
mode, may be disturbed by the coupling or excitation of untuned
modes, causing heating, noise, inadequate vibration amplitudes,
low reliability and even component failures [6,7].
The complexity of the structure of the plate transducers, which
are high modal density systems and combine longitudinal and ex-
Fig. 11. Comparison of amplitude distribution between at and slightly grooved rectangular plates.
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the propagation medium. For ultrasonic radiation in air the wavelength is shorter than 23 cm, but for radiation in water the wavelength is ve times longer. The design of directional stepped-plates
for radiation in water results impractical at low ultrasonic frequencies due to the high height required for the steps. Solutions to obtain directional radiation in liquids (or in air at sonic frequencies)
without using steps have been studied. As a result, a new type of
vibrating plate transducer has been designed and constructed.
The objective is to obtain a high directional radiation with a feasible and easily repeatable construction. In addition, the new transducers have the important novelty of using the radiation of both
faces of the vibrating plate. This is a very important point because
it is equivalent to double the efciency of the transducer.
The idea behind the new design is again to put in phase the
radiation which is emitted by plate zones vibrating in counterphase. However, the use of the radiation from both plate faces implies to bear in mind that the emission from one specic plate sector is in counter-phase at both sides of the plate.
The procedure consists of separating the radiation of each internodal sector by means of parallel walls which are perpendicular to
the plate surface and exactly located in the nodal lines, without
touching the plate. These walls constitute a kind of channels which
are closed by a reector forming 45 with the radiating surface
(Fig. 14). The distance from the reector to the surface of the radiating plate differs for the sectors vibrating in counter-phase just in
half a wavelength of the radiation (k/2). In such a way the radiation
generated by the exural vibrating plate and reected by the
reectors placed alternatively at distances l and l + k/2, is emerging
all in phase on a perpendicular plane to the plate. To be noted that
the reectors on both sides of a same plate sector are placed at distances differing in k/2 [12].
Following the above explained procedure, a transducer prototype was constructed with a rectangular plate radiator for operation in air at a frequency of 9.7 kHz. Fig. 15 shows a photograph
of the prototype. The plate is driven at its centre in similar way
to the other plate transducers. The high directional radiation obtained with the prototype (Fig. 16) conrms the good performance
of the new transducer.
3.5. The transducer with cylindrical radiator
For applications where an intense ultrasonic eld inside a treatment chamber is required, the own chamber can be used as ultrasonic radiator. In this way, a transducer with a cylindrical radiator
has been conceived and developed. The transducer has the same
general structure showed in Fig. 1 but the radiator is a cylinder instead of a plate. The cylinder is driven in one of its exural modes.
In the prototype shown in Fig. 17 the cylindrical radiator vibrates
with twelve nodal lines at a frequency of 21 kHz. The vibration
modes of the cylindrical chamber were studied by using nite element (FE) simulation.
The acoustic eld inside the tube was also computed by FE and
experimentally validated. For a power applied to the transducer of
about 75 W, an average sound pressure level of about 153 dB is obtained inside the cylindrical chamber (Fig. 18). Therefore, a high level acoustic eld is generated with a relatively low power applied
[13].
4. The use of the transducers in industrial processes
The introduction of the new family of transducers with extensive radiators has signicantly contributed to the implementation
at semi-industrial and industrial level of a number of processes
in food industry, in environment and in manufacturing. The different types of transducers previously described were conceived and
designed bearing in mind the needs of specic applications. This is
an important feature to be considered for the right development of
the HPU industrial applications.
This section deals with a summary of such HPU processes,
underlining the role of the type of transducer employed.
4.1. HPU transducers in food industry
Fig. 14. Scheme for the design of a at-plate radiator with reectors.
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ity, but is expensive. Ultrasonic dehydration performed by applying the new transducers via air-borne radiation or in direct contact
with food products, has been proven to be an attractive alternative
for separating moisture from food.
The drying procedure by air-borne ultrasound together with
forced-air has been developed in two different techniques: (a) by
applying the directional stepped-plate ultrasonic transducer and
(b) by applying the transducer with cylindrical radiator as a uidized bed dryer.
In the drying system with the stepped-plate directional transducer, a high-intensity standing wave eld is generated with the
sample holder acting as a reector and it is combined with
forced-air at different temperatures. The high directivity of the
transducer allows the proper formation of the standing wave eld
and consequently high pressure levels (155160 dB) are obtained.
The effect of the ultrasonic radiation with forced-air is signicant
at air temperatures up to about 60 C and diminishes when temperature increases. Hence the application of air-borne ultrasound
is useful to increase the efciency of forced-air drying processes
at temperatures under about 80 C.
In the application of the cylindrical radiator transducer as a uidized bed dryer, the conventional uidized bed drying chamber is
replaced by the vibrating cylinder which constitutes the radiator of
the transducer generating a high-intensity ultrasonic eld in its inside. The uidized bed dryer assisted by ultrasound has shown to
be effective, especially with particulate material.
Ultrasonic dehydration by applying high-intensity ultrasonic
vibration in direct contact with the food material is implemented
by using grooved-plate transducers of rectangular shape. The good
acoustic impedance matching between the vibrating at face of the
plate transducer and the food material signicantly increases the
energy transfer and consequently the effectiveness of the drying
process. The procedure has shown to be commercially interesting
both for its high efciency and for the good preservation of the
food quality. It has been implemented in a full drying system currently at semi-industrial stage.
4.2. HPU transducers in environmental processes
Power ultrasound is a technology that offers several important
possibilities to act as an efcient tool in processes for preventing
or removing pollution. Air cleaning and sludge ltration are two
processes developed by using the new power transducers.
High-power ultrasonic processing may be effective in the release of the residual moisture. Ultrasonic energy directly coupled
to the sludge causes alternating stresses that make an effective
deliquoring by creating a kind of sponge effect and channels
for moisture migration.
A power ultrasonic transducer with a rectangular grooved-plate
radiator has been associated to a conventional rotary vacuum ceramic lter for sludge ltration. The transducer is applied directly
coupled to the cake formed into the lter surface during the process. The effect of the application of ultrasonic energy has shown
that an additional dewatering of about 25% of the residual interstitial moisture can be obtained with a short treatment time (2 s) and
a relatively low power applied (60 W). Such result represents a signicant improvement because the conventional lters are not able
to remove such moisture.
4.3. HPU transducers in manufacturing processes
The versatility of the ultrasonic energy allows it to be used in
many different manufacturing processes usually as an additional
tool to improve either the manufactured product or the process.
By using the new transducers, three different manufacturing processes have been developed.
4.3.1. Ultrasonic washing in textile manufacture [24,25]
Fabric processing in textile manufacturing is a wet processing
that usually requires washing the fabric. The use of ultrasonic energy in such operations may help in speeding up the process and in
improving the quality of the nal product.
A new procedure has been developed by applying rectangular
grooved-plate transducers. The textiles are submerged in a layer
of liquid of a few millimeters in thickness and conveyed in a at
format at a continuous speed through the ultrasonic radiator by
means of a roller-type system. The plate radiator is designed to vibrate with one of its simpler exural vibration modes to avoid
great differences in the vibration amplitudes of the different areas
of the plate and, consequently, to produce as much as possible a
homogeneous cavitation eld in front of the surface of the plate
radiator. The washing performance achieved at a speed of about
2 cm/s and relatively moderate acoustic intensities is clearly much
higher and quicker than that obtained with a conventional washing machine and the energy consumption is very low (of the order
of 0.1 kWh/ kg of textile). Such process has been implemented at
semi-industrial stage.
4.3.2. Ultrasonic debubbling of liquid coating layers [26,27]
Industrial coatings applied at high speed often contain bubbles
from air entrapped during operation. Such bubbles will produce
permanent surface defects after drying and, consequently, piece
rejections in the production line. Chemical additives are generally
used to alleviate the problem, but they are difcult to dose and, if
not properly handled, can create problems which may be even
worse than the air retention.
High-intensity air-borne ultrasound represents an adequate
contact-less method to break the bubbles. A new process based
on the direct application of air-borne ultrasound by using directional stepped-plate transducers has been developed to break the
bubbles which are semi-submerged within the coating layer. Such
process has been implemented at laboratory and semi-industrial
stages.
4.3.3. Ultrasonic enhancement of pigment dispersion in paint
manufacture [28]
Paint is a dispersion of small, coloured, insoluble particles (pigments) in a liquid medium composed of solvent and binder. Pigments are very ne powders that provide colour and the ability
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to hide the underline surface. Most of the paint properties are enhanced when the pigment particles are the smallest possible. Good
pigment dispersion is a critical factor in the manufacture of paint
because it is a complicated and cost-intensive operation. The
objective of dispersion is to incorporate homogeneously particles
into a liquid system, to disagglomerate the pigment powder, to stabilize this dispersion and to assure that it remains stable during
drying.
The application to this processing problem of a new technology
based on power ultrasound offers a potential of innovation which
is required in the paint industry. In fact, ultrasonic energy is a powerful dispersion tool as it can disagglomerate by cavitation pigment
clusters at the microscopic scale, a scale which is impossible to
reach with the conventional industrial equipment.
By using rectangular grooved-plate power ultrasonic transducers, an ultrasonic reactor to enhance pigment dispersion in paints,
pastes and inks at semi- industrial scale has been developed. In
such reactor the generation of ultrasound is provided by three
transducers, mounted in line and in a closed chamber. They produce strong cavitation in a volume around the plate radiators
which are placed inside a chamber where the paint ows.
Trials performed with the prototype of ultrasound machine,
sonicating with applied powers to the transducers in the range of
400600 W and treating paint ows of 50100 kg/h, proved the
pigment disagglomeration effect and that better pigment dispersion can be obtained than with classical grinding machines. Industrial equipments for paint manufacture will require further
development by applying transducers with higher power capacity.
5. Conclusion
The new family of power transducers with extensive radiators
presented in this paper represent an efcient group of ultrasonic
generators for industrial processing in uids and multi-phase media. The technological versatility and effectiveness of such devices
have been proven in a wide range of processes at semi-industrial
and/or industrial scale. Hence, their extended use for large-scale
industrial applications will signify a major breakthrough in HPU
technology.
Acknowledgments
The authors are very grateful to Alberto Pinto and Ignacio Martinez for their technical assistance in many of the developments
presented in this article and to Florence Buisson for her help in
the preparation of this manuscript.
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