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2 authors:
[http://dx.doi.org/10.1063/1.4812588]
The collective excitations of quantum plasmas with the elec- Electron number density and mass are ne and me, respec-
tron exchange and electron-correlations potentials induce a tively. The third term of Eq. (3) is the so-called Bohm
frequency-shift.16 The quantum mechanical correction to the potential. Mostly, in expansion problem, the density decays
electron-ion collision frequency at high temperatures in with a profile close to an exponential function, that the
plasma is found to increase the electron temperature.17 Mola Bohm potential can be neglected. Moreover, this potential
et al. investigated the expansion of a quantum electron gas term could be comparable to the Fermi pressure force term
via the one-particle Schr€odinger-Poisson model. Based on when the density is low and the wavelength is short such as
rescaling methods, they found that the quantum asymptotic in semiconductor plasmas23 but negligible compared to
solution is identical to the classical one.18 the degeneracy pressure term.24 The exchange-correlation
Recently, the first experiment with x-ray laser of kiloelec- potential Vxc arises due to the exchange-correlation forces
tronvolt (keV) photon energy was reported. The observations between the identical particles when their wave functions
of photoabsorption mechanisms and femtosecond electronic overlap due to their high number density. This potential is
response in a prototypical atom of ultra-intense, short-wave- given by25
length regime showed that sequential single-photon absorp- " #
tion dominates and any process that is energetically feasible e2 1=3 0:034 1=3
with a single photon is observed. The photoabsorption mecha- Vxc ¼ 0:985 ne 1 þ 1=3
ln½1 þ 18:37aB ne ; (4)
a ne B
nism at high x-ray intensity is expected to produce plasma
with degenerate electrons by multiple photons absorption.19
In the present paper, the expansion of plasma with single where aB ¼ h2 =me e2 is the Bohr radius, ¼ o r the dielec-
ion species and degenerate electrons is investigated using a tric permittivity of the material, and h the Planck constant
self-similar approach. The effects of the electron-exchange divided by 2p.
and electron-correlations on the plasma expansion are stud- At high-densities, the electrons are degenerate with a
ied in the aim to understand the expansion mechanisms of pressure, in the non-relativistic limit case, given by26,27
strongly coupled plasma states. The latter correspond to
pe ¼ Kncee ; (5)
short-living, highly excited states of matter, near-solid den-
sity plasma states which are an area of active research.20
with
II. MODELING 1
5 5 p 3 ph2
The interaction of a femto-second laser pulses with ce ¼ and K ¼ : (6)
3 3 3 me
planar targets generates plasmas in warm dense matter
regime at near solid-density. The plasma expands perpendic-
We shall combine the basic set of fluid equations (1)–(5)
ular to the target surface onto the target as well as outward.21
to obtain ordinary differential equations using a self-similar
The latter expansion is studied in one-dimension by two
approach. A phenomenon is called self-similar, if the spatial
fluids model, inertialess degenerate electrons and inertial
distributions of its properties at different periods of time can
ions. Due to electron-ion strong correlations, the expansion
be obtained from one another by a similarity transformation.
is mainly driven by the electrostatic potential /. However,
This implies that the local scale length ni =ð@ni =@xÞ is much
for high density plasma, the pressure term cannot be
larger than the Debye length kD ¼ ½o =eðdne =d/Þ, i.e., a
neglected. The ion fluid equations are
quasi-neutral expansion.28 The self-similar approach reduces
@ni @ the set of partially differential equations to an ordinary one.
þ ðni vi Þ ¼ 0; (1) Thus, the moving boundary problem could be overpassed by
@t @x
using initial boundary conditions. The self-similar solution is
@vi @vi e @/ 1 @pi an asymptotic solution valid for large values of time.29 In
þ vi ¼ ; (2)
@t @x mi @x mi ni @x quantum plasmas, the analog of the Debye length is the
Thomas-Fermi length kF ¼ vF =xp , where vF is the Fermi
where ni and vi stand for the ion number density and the ion electron speed and xp the electron plasma frequency. We
velocity, respectively, mi and e are the ion mass and the mag- note that kF describes the scale length of the electrostatic
nitude of the electron charge, respectively. For an adiabatic screening of ions by degenerate electrons in a quantum
expansion, the ion pressure depends on the polytropic coeffi- plasma.30
c
cient ci , and pi ni i ¼ Constant. The set of governing equations is transformed using the
In warm dense matter of temperature ranging from self-similar variable n ¼ x=t. The latter has the dimension
0.1 eV to several eV, quantum effects are important when of velocity. It is worth to note that, in general, the set of dif-
the density is of the order of 1023 cm3 (c.f. Ref. 22). The ferential equations are transformed using a dimensionless
inertialess degenerate electron fluids momentum equation is variable n ¼ x=Cs t, if the ion-acoustic speed Cs is known.31
given by In the present study, the Fermi ion-acoustic speed has to be
calculated under the combined influence of the quantum
" pffiffiffiffiffi#
@/ @Vxc h2 @ 1 @ 2 ne 1 @pe statistical pressure, as well as the electron-exchange and
e þ pffiffiffiffiffi 2
¼ 0: (3) electron-correlations effects on the dynamics of degenerate
@x @x 2me @x ne @x ne @x
electrons.
072702-3 M. Djebli and W. M. Moslem Phys. Plasmas 20, 072702 (2013)
A. The Fermi acoustic speed As the expansion occurs in the positive x direction, the plus
sign is more appropriate.
At the expanding front, during the beginning of the
expansion, a disturbance creates a region of compressed par-
ticles that is pushing in the front creating a rarefaction wave III. DISCUSSION
behind. The speed, at which this disturbance propagates, is
The expansion front is formed by some of the ions that
known as the Fermi acoustic speed. The Fermi acoustic
are subsequently accelerated, and is associated with density
wave associated to this speed governs the evolution of the
depletion. The region of decreasing density moves into the
mass density due to the pressure gradient, charge imbalance
ambient plasma at the ion-acoustic speed. First, let us focus
and characterize the time scale of the phenomenon under
on an isothermal plasma expansion (ci ¼ 1). For classical
investigation.
plasmas when both electrons and ions are non-degenerate,
We close the set of differential equations (1)–(5) by
the finite expansion studied in the limit of half space expan-
invoking the quasi-neutrality assumption ne ¼ ni . As the
sion occurs with velocity following a linear profile. Initially,
density of particles in the plasma region is very high, the
the plasma is supposed to fill the half space x < 0 and the
space scale associated with Poisson’s equation is very
front is moving with the same velocity as the ion-acoustic
small.32 Therefore, the quasi-neutrality assumption can be
speed Cs, the time scale corresponds to the ion motion. The
used and turns out to make numerical solution possible by
electric field is space independent and is different from zero
invoking an appropriate self-similar transformation given by
when x ! 0. When the expansion starts with an unperturbed
the ans€atze
plasma (nðno Þ ¼ no ), ions located at the discontinuity x ¼ 0
mi are accelerated to infinity by the infinite electric field as soon
ni ¼ Nno ; /¼ U; pi ¼ mi no P: (7)
e as t > 0, the ion velocity increases linearly along the x axis
for a given t.8,33 From Eq. (13), the Fermi acoustic speed
By using Eqs. (4), (5), and the ion equation of state, in terms depends on the quantum parameters. To investigate the prop-
of the self-similar variable n, yield to a set of ordinary differ- erties of plasma expansion in the presence of quantum
ential equations governing the expansion effects, we numerically solve Eqs. (11) and (12) to follow
the expansion front in terms of the self-similar variable,
dN dv
ðv nÞ þN ¼ 0; (8) then the evolution of the acoustic speed can be obtained.
dn dn Numerical discretization is based on Euler scheme, this
dv dU dN method is used instead of Rung-Kutta or other algorithms
ðv nÞ ¼ rN c2 ; (9) because it is very stable. The desired accuracy is achieved by
dn dn dn
choosing a very small step to implement iterations. These
dU dN dN bN 2=3 dN approaches are motivated by the difficulties in following the
¼ dN ðce 1Þ aN 2=3 : (10)
dn dn dn 1 þ N 1=3 dn plasma-vacuum interface where numerical instabilities can
grow.34 Our plasma model is inspired by solid-density plas-
Then, Eq. (10) is used to eliminate the electrostatic potential mas. Hence, our results are applied to a beryllium plasma
from Eq. (9) to obtain produced by a femto-second laser interaction with planar tar-
gets.21,35 The main contribution of the quantum mechanical
dN dv effects comes from the coefficients a, b, and , which are
ðv nÞ þN ¼0 (11)
dn dn depending on the relative dielectric permittivity. In the case
of the beryllium plasma near solid-density, the relative per-
and mittivity varies within the range [5, 15].36 Three cases
" # are investigated ¼ 5; 10, and 15 with typical parameters
dv bN 2=3
ðv nÞ þ rN ðci 2Þ
þ dN ðce 2Þ
þ aN 2=3
þ n0 ¼ 2 1023 cm3 and To Te ¼ 12 eV. Relying on the
dn ð1 þ N 1=3 Þ above typical physical parameters, we have numerically
dN investigated the properties of the Fermi ion-acoustic speed
¼ 0; ð12Þ Cs, as depicted in Figs. 1(a), the dependence of the Fermi
dn
ion-acoustic speed Cs on the perturbed ion number density N
where no is the plasma density at equilibrium. We have is considered. Comparing this figure with the expansion of
dropped the subscript i, that v ¼ vi . The constants are classical plasmas, the acoustic speed is depending upon the
a ¼ 0:985e2 no1=3 =3m; b ¼ 0:034 18:37a; d ¼ ce Knoðce 1Þ =me , density. We note that N ¼ 1 corresponds to the start of the
and r ¼ ce To =m and ¼ 18:37aB no1=3 . The expansion is expansion. In the isothermal process, the plasma is supposed
assumed to start from an unperturbed plasma characterized to be connected to a thermal reservoir. As the electron corre-
by the ion number density no and the ion temperature To. lation effect is considered, it is not possible to recover the
From Eqs. (11) and (12), one obtains the front ion speed classical plasma result, i.e., the acoustic speed is independent
of the medium density, by putting r ¼ 1. The Fermi ion
v ¼ n6Cs
qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi acoustic speed reflects the interaction of the ion wave with
¼ n6 rN ðci 1Þ þ dN ðce 1Þ þ aN 1=3 þ bN 1=3 =ð1 þ N 1=3 Þ: the electrostatic fields of the plasma positive charges. This
interaction is more important when the correlations are stron-
(13) ger. For higher r , the plasma behaves as a solid with an
072702-4 M. Djebli and W. M. Moslem Phys. Plasmas 20, 072702 (2013)
acoustic speed, in more dense materials the acoustic wave is quantum mechanical effects are significant for plasmas near
transmitted slower. Moreover, the acoustic speed defines the solid density. The reduction of the medium density is associ-
time scale of the expansion. In the presence of degenerate ated with an oscillation region at the expanding front, which
electrons, the ion acceleration is found to be higher by a becomes reduced and finite leading to the formation of a
factor of 105 order. rarefaction shock. The latter effect increases the local charge
For the adiabatic plasma expansion, higher values of the separation between ions and electrons which in turns weaken
acoustic speed are observed for lower values of the relative the effect of electron correlation.
permittivity (Fig. 1(b)). When the density decreases, the One of the problems related to the plasma expansion is
acoustic speed decreases, but faster with an abrupt fall the choice of the initial velocity, taken here vðn ¼ no Þ ¼ 0,
when ni 0:1no . By lowering the initial density, we recover when the expansion is supposed to start with an unperturbed
the classical case, i.e., the plasma expansion with non- plasma. It is well known that the expansion results from the
degenerate electrons, the acoustic speed depends only on the combination of the thermal pressure and the ambipolar elec-
density and the polytropic exponent (Cs ¼ ci nci 1 ).8 This can trostatic potential. In addition, in the presence of degenerate
be seen when no 1019 cm3 (Figs. 2(a) and 2(b)). Thus, the electrons, there is a gradient of degenerate electron pressure,
as well a gradient of potentials associated with an electron- indefinitely, it losses its physical meaning when the density
exchange potential and electron-correlations. In Figs. 3(b) vanishes ðN 0Þ (Figs. 3(a) and 3(c)). Moreover, the adia-
and 3(d) are plotted the density and velocity for two different batic expansion is associated to ions cooling effect, making
ion initial temperature T0 Te ¼ 12 eV (black lines) and the adiabatic expansion ends earlier than the isothermal
1 eV (red lines) with relative permittivity r ¼ 1 (solid lines) expansion (comparison is made between dashed black lines).
and 15 (dashed lines). The velocity almost keeps its linear The isothermal expansion supposes that the plasma is con-
profile in the isothermal case (Fig. 3(b)). The ion accelera- nected to some energy reservoir. Thus, smaller limit for the
tion can be depicted for both isothermal and adiabatic cases. self-similar parameter means that the expansion is held in a
For the adiabatic case, the velocity becomes independent shorter time or ends very close to the plasma source region.
from the density far away from the plasma source region and In large-size systems, the charged particles can be considered
reaches the same limit which depends on the relative permit- far away from each other, so that one can assume that the
tivity (solid and dashed lines). The lower permittivity is the potential varies slowly on the scale given by the size of
higher the velocity is. We can conclude that the quantum the charge distribution, and the adiabatic process remains the
effects are more important close to the plasma source region same. This can be used as a first approximation, which
where the density is high. Far away from the source region, allows a set of conservation laws.37 It turns out that for the
the ambipolar potential is the main mechanism that governs plasma produced by high intensity-laser with a light
the plasma expansion. Since the velocity cannot increase weight metallic target, adiabatic expansion profiles offer a
4
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